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  Mechanisms for Long-Lived, Photo-Induced Superconductivity

Chattopadhyay, S., Eckhardt, C., Kennes, D. M., Sentef, M. A., Shin, D., Rubio, A., et al. (2023). Mechanisms for Long-Lived, Photo-Induced Superconductivity.

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2303.15355.pdf (Preprint), 2MB
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2303.15355.pdf
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File downloaded from arXiv at 2023-03-28
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2023
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https://arxiv.org/abs/2303.15355 (Preprint)
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 Urheber:
Chattopadhyay, S.1, Autor
Eckhardt, C.2, 3, 4, Autor           
Kennes, D. M.2, 4, 5, Autor           
Sentef, M. A.3, 4, 6, Autor           
Shin, D.4, 5, 7, Autor           
Rubio, A.4, 5, Autor           
Cavalleri, A.4, 8, 9, Autor           
Demler, E. A.10, Autor
Michael, M.4, 5, Autor           
Affiliations:
1Lyman Laboratory, Department of Physics, Harvard University, ou_persistent22              
2Institut für Theorie der Statistischen Physik, RWTH Aachen University and JARA-Fundamentals of Future Information Technology, ou_persistent22              
3Theoretical Description of Pump-Probe Spectroscopies in Solids, Theory Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_3012828              
4Center for Free-Electron Laser Science (CFEL), ou_persistent22              
5Theory Group, Theory Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_2266715              
6H H Wills Physics Laboratory, University of Bristol, ou_persistent22              
7Gwangju Institute of Science and Technology, ou_persistent22              
8Quantum Condensed Matter Dynamics, Condensed Matter Dynamics Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_1938293              
9Department of Physics, Clarendon Laboratory, University of Oxford, ou_persistent22              
10Institute for Theoretical Physics, ETH Zürich, ou_persistent22              

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Schlagwörter: Condensed Matter, Superconductivity, cond-mat.supr-con, Condensed Matter, Mesoscale and Nanoscale Physics, cond-mat.mes-hall, Condensed Matter, Statistical Mechanics, cond-mat.stat-mech, Condensed Matter, Strongly Correlated Electrons, cond-mat.str-el, Physics, Optics, physics.optics
 Zusammenfassung: Advances in the control of intense infrared light have led to the striking discovery of metastable superconductivity in K3C60 at 100K, lasting more than 10 nanoseconds. Inspired by these experiments, we discuss possible mechanisms for long-lived, photo-induced superconductivity above Tc. We analyze a minimal model of optically-driven Raman phonons coupled to inter-band electronic transitions. Using this model, we develop a possible microscopic mechanism for photo-controlling the pairing interaction by displacively shifting the Raman mode. Leveraging this mechanism, we explore two pictures of long-lived, light-induced superconductivity far above Tc. We first investigate long-lived, photo-induced superconductivity arising from the metastable trapping of a displaced phonon coordinate. We then propose an alternate route to long-lived superconductivity. Within this paradigm, the slow equilibration of quasi-particles enables a long-lived, non-thermal superconducting gap. We conclude by discussing implications of both scenarios to experiments that can be used to discriminate between them. Our work provides falsifiable, mechanistic explanations for the nanosecond scale photo-induced superconductivity found in K3C60, while also offering a theoretical basis for exploring long-lived, non-equilibrium superconductivity in other quantum materials.

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Sprache(n): eng - English
 Datum: 2023-03-27
 Publikationsstatus: Online veröffentlicht
 Seiten: 18
 Ort, Verlag, Ausgabe: -
 Inhaltsverzeichnis: -
 Art der Begutachtung: Keine Begutachtung
 Identifikatoren: arXiv: 2303.15355
 Art des Abschluß: -

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