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  Extended regime of metastable metallic and insulating phases in a two-orbital electronic system

Vandelli, M., Kaufmann, J., Harkov, V., Lichtenstein, A. I., Held, K., & Stepanov, E. A. (2023). Extended regime of metastable metallic and insulating phases in a two-orbital electronic system. Physical Review Research, 5(2): L022016. doi:10.1103/PhysRevResearch.5.L022016.

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PhysRevResearch.5.L022016.pdf (Verlagsversion), 503KB
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2023
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© the Author(s). Published by the American Physical Society
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Supplemental Material: Detailed discussion of the hysteresis curve and calculations for a non-zero value of the Hund's coupling.
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https://doi.org/10.1103/PhysRevResearch.5.L022016 (Verlagsversion)
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 Urheber:
Vandelli, M.1, 2, 3, 4, 5, Autor           
Kaufmann, J.6, Autor
Harkov, V.1, 7, Autor
Lichtenstein, A. I.1, 2, 7, Autor
Held, K.6, Autor
Stepanov, E. A.8, Autor
Affiliations:
1I. Institute of Theoretical Physics, University of Hamburg, ou_persistent22              
2The Hamburg Centre for Ultrafast Imaging, ou_persistent22              
3Theory Group, Theory Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_2266715              
4Center for Free-Electron Laser Science, ou_persistent22              
5International Max Planck Research School for Ultrafast Imaging & Structural Dynamics (IMPRS-UFAST), Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_2266714              
6Institute of Solid State Physics, ou_persistent22              
7European X-Ray Free-Electron Laser Facility, ou_persistent22              
8CPHT, CNRS, École polytechnique, Institut Polytechnique de Paris, ou_persistent22              

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 Zusammenfassung: We investigate the metal-to-insulator phase transition driven by the density-density electronic interaction in the quarter-filled model on a cubic lattice with two orbitals split by a crystal field. We show that a systematic consideration of the nonlocal collective electronic fluctuations strongly affects the picture of the phase transition provided by the dynamical mean-field theory. Our calculations reveal the appearance of metallic and Mott insulating states characterized by the same density but different values of the chemical potential, which is missing in the local approximation to electronic correlations. We find that the region of concomitant metastability of these two solutions is remarkably broad in terms of the interaction strength. It starts at a critical value of the interaction slightly larger than the bandwidth and extends to more than twice the bandwidth, where the two solutions merge into a Mott insulating phase. Our results illustrate that nonlocal correlations can have crucial consequences on the electronic properties in the strongly correlated regime of the simplest multiorbital systems.

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Sprache(n): eng - English
 Datum: 2023-02-162022-04-052023-02-172023-04-25
 Publikationsstatus: Online veröffentlicht
 Seiten: -
 Ort, Verlag, Ausgabe: -
 Inhaltsverzeichnis: -
 Art der Begutachtung: Expertenbegutachtung
 Identifikatoren: DOI: 10.1103/PhysRevResearch.5.L022016
 Art des Abschluß: -

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Projektname : M.V., V.H., and A.I.L. acknowledge the support by the Cluster of Excellence “Advanced Imaging of Matter” of the Deutsche Forschungsgemeinschaft (DFG) - EXC 2056 - Project No. ID390715994, and by North-German Supercomputing Alliance (HLRN) under Project No. hhp00042. J.K. and K.H. have been supported by the Austrian Science Fund (FWF) through Projects No. P32044 and No. I5868 (“Quast”). V.H. and A.I.L. further acknowledge the support by the DFG through FOR 5249-449872909 (Project No. P8) and the European Research Council via Synergy Grant No. 854843-FASTCORR. The work of E.A.S. was supported by the European Union's Horizon 2020 Research and Innovation programme under the Marie Skłodowska Curie Grant Agreement No. 839551 - 2DMAGICS. E.A.S. is also thankful to the CPHT computer support team.
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Titel: Physical Review Research
Genre der Quelle: Zeitschrift
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Ort, Verlag, Ausgabe: College Park, Maryland, United States : American Physical Society (APS)
Seiten: - Band / Heft: 5 (2) Artikelnummer: L022016 Start- / Endseite: - Identifikator: ISSN: 2643-1564
CoNE: https://pure.mpg.de/cone/journals/resource/2643-1564