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  Interplay between Magnetism and Topology: Large Topological Hall Effect in an Antiferromagnetic Topological Insulator, EuCuAs

Roychowdhury, S., Samanta, K., Yanda, P., Malaman, B., Yao, M., Schnelle, W., et al. (2023). Interplay between Magnetism and Topology: Large Topological Hall Effect in an Antiferromagnetic Topological Insulator, EuCuAs. Journal of the American Chemical Society, 145(23), 12920-12927. doi:10.1021/jacs.3c04249.

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Roychowdhury, Subhajit1, Autor
Samanta, Kartik2, Autor           
Yanda, Premakumar2, Autor           
Malaman, Bernard1, Autor
Yao, Mengyu2, Autor           
Schnelle, Walter3, Autor           
Guilmeau, Emmanuel1, Autor
Constantinou, Procopios1, Autor
Chandra, Sushmita2, Autor           
Borrmann, Horst4, Autor           
G. Vergniory, Maia2, Autor           
Strocov, Vladimir1, Autor
Shekhar, Chandra5, Autor           
Felser, Claudia6, Autor           
Affiliations:
1External Organizations, ou_persistent22              
2Inorganic Chemistry, Max Planck Institute for Chemical Physics of Solids, Max Planck Society, ou_1863425              
3Walter Schnelle, Inorganic Chemistry, Max Planck Institute for Chemical Physics of Solids, Max Planck Society, ou_1863441              
4Horst Borrmann, Chemical Metal Science, Max Planck Institute for Chemical Physics of Solids, Max Planck Society, ou_1863410              
5Chandra Shekhar, Inorganic Chemistry, Max Planck Institute for Chemical Physics of Solids, Max Planck Society, ou_1863428              
6Claudia Felser, Inorganic Chemistry, Max Planck Institute for Chemical Physics of Solids, Max Planck Society, ou_1863429              

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 Zusammenfassung: Magnetic interactions in combination with nontrivial band structures can give rise to several exotic physical properties such as a large anomalous Hall effect, the anomalous Nernst effect, and the topological Hall effect (THE). Antiferromagnetic (AFM) materials exhibit the THE due to the presence of nontrivial spin structures. EuCuAs crystallizes in a hexagonal structure with an AFM ground state (Neel temperature similar to 16 K). In this work, we observe a large topological Hall resistivity of similar to 7.4 mu Omega-cm at 13 K which is significantly higher than the giant topological Hall effect of Gd2PdSi3 (similar to 3 mu Omega-cm). Neutron diffraction experiments reveal that the spins form a transverse conical structure during the metamagnetic transition, resulting in the large THE. In addition, by controlling the magnetic ordering structure of EuCuAs with an external magnetic field, several fascinating topological states such as Dirac and Weyl semimetals have been revealed. These results suggest the possibility of spintronic devices based on antiferromagnets with tailored noncoplanar spin configurations.

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Sprache(n): eng - English
 Datum: 2023-06-022023-06-02
 Publikationsstatus: Erschienen
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 Ort, Verlag, Ausgabe: -
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 Art der Begutachtung: -
 Identifikatoren: ISI: 001008284400001
DOI: 10.1021/jacs.3c04249
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Titel: Journal of the American Chemical Society
  Andere : JACS
  Kurztitel : J. Am. Chem. Soc.
Genre der Quelle: Zeitschrift
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Ort, Verlag, Ausgabe: Washington, DC : American Chemical Society
Seiten: - Band / Heft: 145 (23) Artikelnummer: - Start- / Endseite: 12920 - 12927 Identifikator: ISSN: 0002-7863
CoNE: https://pure.mpg.de/cone/journals/resource/954925376870