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  Hyperthermal velocity distributions of recombinatively-desorbing oxygen from Ag(111)

Dorst, A. C., Dissanayake, R. E. A., Schauermann, D., Knies, S., Wodtke, A. M., Killelea, D., et al. (2023). Hyperthermal velocity distributions of recombinatively-desorbing oxygen from Ag(111). Frontiers in Chemistry, 11: 1248456. doi:10.3389/fchem.2023.1248456.

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Item Permalink: https://hdl.handle.net/21.11116/0000-000D-BFCD-6 Version Permalink: https://hdl.handle.net/21.11116/0000-000D-BFCE-5
Genre: Journal Article

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fchem-11-1248456.pdf (Publisher version), 2MB
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 Creators:
Dorst, Arved Cedric1, Author           
Dissanayake, Rasika E. A.1, Author           
Schauermann, D., Author
Knies, S., Author
Wodtke, Alec M.1, Author                 
Killelea, D.R., Author
Schäfer, Tim1, Author           
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1Department of Dynamics at Surfaces, Max Planck Institute for Multidisciplinary Sciences, Max Planck Society, ou_3350158              

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 Abstract: This study presents velocity-resolved desorption experiments of recombinatively-desorbing oxygen from Ag (111). We combine molecular beam techniques, ion imaging, and temperature-programmed desorption to obtain translational energy distributions of desorbing O2. Molecular beams of NO2 are used to prepare a p (4 × 4)-O adlayer on the silver crystal. The translational energy distributions of O2 are shifted towards hyperthermal energies indicating desorption from an intermediate activated molecular chemisorption state.

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Language(s): eng - English
 Dates: 2023-08-022023
 Publication Status: Issued
 Pages: -
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 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.3389/fchem.2023.1248456
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Project name : TS acknowledges support from the Deutsche Forschungsgemeinschaft (DFG) under grant SCHA 1946/5-1 and INST 186/1302-1 and support from the Deutscher Akademische Austauschdienst (DAAD) (Grant 57651434). RD acknowledges funding under a Georg Forster research fellowship from the Humboldt foundation. DK acknowledges support from the National Science Foundation through award CHE-2155068 and ICASEC at University of Göttingen.
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Title: Frontiers in Chemistry
  Abbreviation : Front. Chem.
Source Genre: Journal
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Publ. Info: Lausanne, Switzerland : Frontiers Media
Pages: - Volume / Issue: 11 Sequence Number: 1248456 Start / End Page: - Identifier: ISSN: 2296-2646
CoNE: https://pure.mpg.de/cone/journals/resource/2296-2646