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  X-ray photoelectron spectroscopy of gaseous and solid I2: Ion-state-enhanced intermolecular interactions

Salaneck, W. R., Bigelow, R. W., Freund, H.-J., & Plummer, E. W. (1981). X-ray photoelectron spectroscopy of gaseous and solid I2: Ion-state-enhanced intermolecular interactions. Physical Review B, 24(5), 2403-2411. doi:10.1103/PhysRevB.24.2403.

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Item Permalink: https://hdl.handle.net/21.11116/0000-000E-A6BF-0 Version Permalink: https://hdl.handle.net/21.11116/0000-000E-A6C0-D
Genre: Journal Article

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PhysRevB.24.2403.pdf (Publisher version), 690KB
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PhysRevB.24.2403.pdf
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1981
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APS
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 Creators:
Salaneck, W. R., Author
Bigelow, R. W., Author
Freund, Hans-Joachim1, Author
Plummer, E. W., Author
Affiliations:
1Physics Department, University of Pennsylvania, Philadelphia, PA, USA, ou_persistent22              

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 Abstract: Gas- and solid-phase x-ray photoelectron spectra of I2 are compared. The shake-up satellite structure on the core-level peaks for I2 in the gas phase can be interpreted using a one-electron model of electronic transitions among states of the molecular ion. In the solid phase, the shake-up transition energies are greatly increased owing to the dynamic nature of the photoionization process, which enhances the intermolecular interactions of the molecular ion with neighboring neutral molecules. Complete-neglect-of-differential-overlap-2 model molecular-orbital calculations have been used to interpret the spectra in terms of strong intermolecular interactions in the solid phase.

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Language(s): eng - English
 Dates: 1981-03-051981-09-01
 Publication Status: Issued
 Pages: 9
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1103/PhysRevB.24.2403
 Degree: -

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Title: Physical Review B
  Abbreviation : Phys. Rev. B
Source Genre: Journal
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Publ. Info: Woodbury, NY : American Physical Society
Pages: 9 Volume / Issue: 24 (5) Sequence Number: - Start / End Page: 2403 - 2411 Identifier: ISSN: 1098-0121
CoNE: https://pure.mpg.de/cone/journals/resource/954925225008