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Electronic properties, Samarium compounds, Tantalum compounds, Temperature distribution, Terahertz waves, Topology, Carrier multiplication, High-field, Linear dispersion, On demands, Property, Resonant condition, Tera Hertz, Terahertz light, Terahertz radiation, Vibrational state, Terahertz spectroscopy
Abstract:
Topological Dirac and Weyl semimetals (D&W SM) have attracted a lot of attention due to their unusual electronic properties, which are strongly dependent on the symmetry of the system. By altering the symmetry of the lattice, using for example a pulse of light, one can expect to modify their topological nature and induce/suppress the related properties 'on demand'. Highfield Terahertz (THz) radiation that interacts with vibrational states under near-resonant conditions is a promising pump candidate to induce structural changes in D&W SM compounds, possibly leading to topological transient or permanent changes. There are, however, some challenges to achieving such control. D&W SM have a specific band structure showing a 3D-linear dispersion around nodes, which makes them sensitive to THz-induced carrier multiplication. These carrier multiplication processes can compete with and ultimately screen the interaction of the THz light with vibrational modes. Here, we present recent results of 2D-THz spectroscopy of a bulk Weyl semimetal TaAs in reflection. We highlight THz-induced carrier multiplication effects and study the field and temperature dependence of the number of carriers induced by the THz field. We examine possible carrier multiplication mechanisms which could be involved. © 2023 IEEE.
