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  Theory of Quantum Light-Matter Interaction in Cavities: Extended Systems and the Long Wavelength Approximation

Svendsen, M. K., Ruggenthaler, M., Hübener, H., Schäfer, C., Eckstein, M., Rubio, A., et al. (2023). Theory of Quantum Light-Matter Interaction in Cavities: Extended Systems and the Long Wavelength Approximation.

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2312.17374.pdf (Preprint), 2MB
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2312.17374.pdf
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https://arxiv.org/abs/2312.17374 (Preprint)
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 Creators:
Svendsen, M. K.1, 2, Author           
Ruggenthaler, M.1, 2, Author           
Hübener, H.1, 2, Author           
Schäfer, C.3, 4, Author
Eckstein, M.5, Author
Rubio, A.1, 2, 6, Author           
Latini, S.1, 7, Author           
Affiliations:
1Theory Group, Theory Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_2266715              
2Center for Free-Electron Laser Science, ou_persistent22              
3Department of Microtechnology and Nanoscience, MC2, Chalmers University of Technology, ou_persistent22              
4Department of Physics, Chalmers University of Technology, ou_persistent22              
5Department of Physics, University Hamburg, ou_persistent22              
6Center for Computational Quantum Physics (CCQ), The Flatiron Institute, ou_persistent22              
7Nanomade, Department of Physics, Technical University of Denmark, ou_persistent22              

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Free keywords: Condensed Matter, Mesoscale and Nanoscale Physics, cond-mat.mes-hall, Physics, Optics, physics.optics,Quantum Physics, quant-ph
 Abstract: When light and matter interact strongly, the coupled system inherits properties from both constituents. It is consequently possible to alter the properties of either by engineering the other. This intriguing possibility has lead to the emergence of the cavity-materials-engineering paradigm which seeks to tailor material properties by engineering the fluctuations of a dark electromagnetic environment. The theoretical description of hybrid light-matter systems is complicated by the combined complexity of a realistic description of the extended electronic and quantum electromagnetic fields. Here we derive an effective, non-perturbative theory for low dimensional crystals embedded in a paradigmatic Fabry-Pérot resonator in the long-wavelength limit. The theory encodes the multi-mode nature of the electromagnetic field into an effective single-mode scheme and it naturally follows from requiring a negligible momentum transfer from the photonic system to the matter. Crucially, in the effective theory the single light mode is characterized by a finite effective mode volume even in the limit of bulk cavity-matter systems and can be directly determined by realistic cavity parameters. As a consequence, the coupling of the effective mode to matter remains finite for bulk materials. By leveraging on the realistic description of the cavity system we make our effective theory free from the double counting of the coupling of matter to the electromagnetic vacuum fluctuations of free space. Our results provide a substantial step towards the realistic description of interacting cavity-matter systems at the level of the fundamental Hamiltonian, by effectively including the electromagnetic environment and going beyond the perfect mirrors approximation.

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Language(s): eng - English
 Dates: 2023-12-28
 Publication Status: Published online
 Pages: 21
 Publishing info: -
 Table of Contents: -
 Rev. Type: No review
 Identifiers: arXiv: 2312.17374
 Degree: -

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