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  High-Order Harmonic Generation in Solids: The Role of Intraband Transitions in Extreme Nonlinear Optics

Hirori, H., Sato, S., & Kanemitsu, Y. (2024). High-Order Harmonic Generation in Solids: The Role of Intraband Transitions in Extreme Nonlinear Optics. The Journal of Physical Chemistry Letters, 15(8), 2184-2192. doi:10.1021/acs.jpclett.3c03415.

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Supporting Information: Microscopic theory of HHG in solids
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 Creators:
Hirori, H.1, Author
Sato, S.2, 3, Author           
Kanemitsu, Y.1, Author
Affiliations:
1Institute for Chemical Research, Kyoto University, ou_persistent22              
2Center for Computational Sciences, University of Tsukuba, ou_persistent22              
3Theory Group, Theory Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_2266715              

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 Abstract: High-order harmonic generation (HHG) in gases is frequently used nowadays to produce attosecond pulses and coherent radiation in the visible-to-soft X-ray spectral range. HHG in solids is a natural extension of the idea of HHG in gases, and its first observation about ten years ago opened the door to investigations on attosecond electron dynamics in solids and the development of solid-state attosecond light sources. The common process in both types of HHG is nonlinear photocarrier generation, and thus, transitions between different bands (interband transitions) are always important for HHG. As well, in the case of solids, the transitions within a band (intraband transitions) also need to be considered, because efficient carrier acceleration is possible due to them. This Perspective focuses on experimental findings that show how intraband transitions can be controlled because such an understanding will be essential in the development of unique optoelectronics that can operate at petahertz frequencies.

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Language(s): eng - English
 Dates: 2024-02-082023-12-052024-02-132024-02-19
 Publication Status: Published online
 Pages: 9
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 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1021/acs.jpclett.3c03415
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Project name : The authors would like to thank many colleagues for their contributions and useful discussions. In particular, the authors gratefully acknowledge K. Nakagawa, Y. Sanari, and T. Yamada for their support. Part of this study was supported by a grant from the Japan Society for the Promotion of Science (JSPS KAKENHI Grant No. JP19H05465). H.H. acknowledges the financial support of the Japan Society for the Promotion of Science (JSPS KAKENHI Grant No. JP21H01842).
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Title: The Journal of Physical Chemistry Letters
  Abbreviation : J. Phys. Chem. Lett.
Source Genre: Journal
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Publ. Info: Washington, DC : American Chemical Society
Pages: - Volume / Issue: 15 (8) Sequence Number: - Start / End Page: 2184 - 2192 Identifier: ISSN: 1948-7185
CoNE: https://pure.mpg.de/cone/journals/resource/1948-7185