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  Electronic Population Reconstruction from Strong-Field-Modified Absorption Spectra with a Convolutional Neural Network

Richter, D., Magunia, A., Rebholz, M., Ott, C., & Pfeifer, T. (2024). Electronic Population Reconstruction from Strong-Field-Modified Absorption Spectra with a Convolutional Neural Network. Optics, 5(1), 88-100. doi:10.3390/opt5010007.

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https://www.mdpi.com/2673-3269/5/1/7 (Publisher version)
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OA-Status:
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 Creators:
Richter, Daniel1, Author           
Magunia, Alexander1, Author                 
Rebholz, Marc1, Author                 
Ott, Christian1, Author                 
Pfeifer, Thomas1, Author                 
Affiliations:
1Division Prof. Dr. Thomas Pfeifer, MPI for Nuclear Physics, Max Planck Society, ou_2025284              

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Free keywords: atomic physics; ultrafast science; electronic population transfer; free-electron laser; transient absorption spectroscopy; extreme ultraviolet light; convolutional neural network
 Abstract: We simulate ultrafast electronic transitions in an atom and corresponding absorption line changes with a numerical, few-level model, similar to previous work. In addition, a convolutional neural network (CNN) is employed for the first time to predict electronic state populations based on the simulated modifications of the absorption lines. We utilize a two-level and four-level system, as well as a variety of laser-pulse peak intensities and detunings, to account for different common scenar- ios of light–matter interaction. As a first step towards the use of CNNs for experimental absorption data in the future, we apply two different noise levels to the simulated input absorption data.

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 Dates: 2024-02-26
 Publication Status: Published online
 Pages: 13
 Publishing info: -
 Table of Contents: -
 Rev. Type: -
 Identifiers: DOI: 10.3390/opt5010007
 Degree: -

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Title: Optics
Source Genre: Journal
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Publ. Info: Schweiz : https://www.mdpi.com/journal/optics
Pages: - Volume / Issue: 5 (1) Sequence Number: - Start / End Page: 88 - 100 Identifier: ISSN: 2673-3269
CoNE: https://pure.mpg.de/cone/journals/resource/2673-3269