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  Observation of Floquet states in graphene

Merboldt, M., Schüler, M., Schmitt, D., Bange, J. P., Bennecke, W., Gadge, K., et al. (2024). Observation of Floquet states in graphene.

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2404.12791.pdf (Preprint), 4MB
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https://arxiv.org/abs/2404.12791 (Preprint)
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 Creators:
Merboldt, M.1, Author
Schüler, M.2, 3, Author
Schmitt, D.1, Author
Bange, J. P.1, Author
Bennecke, W.1, Author
Gadge, K.4, Author
Pierz, K.5, Author
Schumacher, H. W.5, Author
Momeni, D.5, Author
Steil, D.1, Author
Manmana, S. R.4, Author
Sentef, M. A.6, 7, 8, Author           
Reutzel, M.1, Author
Mathias, S.1, 9, Author
Affiliations:
1I. Physikalisches Institut, Georg-August-Universität Göttingen, ou_persistent22              
2Laboratory for Materials Simulations, Paul Scherrer Institute, ou_persistent22              
3Department of Physics, University of Fribourg, ou_persistent22              
4Institut für Theoretische Physik, Georg-August-Universität Göttingen, ou_persistent22              
5Physikalisch-Technische Bundesanstalt, ou_persistent22              
6Institute for Theoretical Physics and Bremen Center for Computational Materials Science, University of Bremen, ou_persistent22              
7Theoretical Description of Pump-Probe Spectroscopies in Solids, Theory Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_3012828              
8Center for Free-Electron Laser Science (CFEL), ou_persistent22              
9International Center for Advanced Studies of Energy Conversion (ICASEC), University of Göttingen, ou_persistent22              

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Free keywords: Condensed Matter, Mesoscale and Nanoscale Physics, cond-mat.mes-hall
 Abstract: Recent advances in the field of condensed-matter physics have unlocked the potential to realize and control emergent material phases that do not exist in thermal equilibrium. One of the most promising concepts in this regard is Floquet engineering, the coherent dressing of matter via time-periodic perturbations. However, the broad applicability of Floquet engineering to quantum materials is still unclear. For the paradigmatic case of monolayer graphene, the theoretically predicted Floquet-induced effects, despite a seminal report of the light-induced anomalous Hall effect, have been put into question. Here, we overcome this problem by using electronic structure measurements to provide direct experimental evidence of Floquet engineering in graphene. We report light-matter-dressed Dirac bands by measuring the contribution of Floquet sidebands, Volkov sidebands, and their quantum path interference to graphene's photoemission spectral function. Our results finally demonstrate that Floquet engineering in graphene is possible, paving the way for the experimental realization of the many theoretical proposals on Floquet-engineered band structures and topological phases.

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Language(s): eng - English
 Dates: 2024-04-19
 Publication Status: Published online
 Pages: 30
 Publishing info: -
 Table of Contents: -
 Rev. Type: No review
 Identifiers: arXiv: 2404.12791
 Degree: -

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