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  Ultrafast Raman thermometry in driven YBa2Cu3O6.48

Chou, T.-H., Först, M., Fechner, M., Henstridge, M., Roy, S., Buzzi, M., et al. (2024). Ultrafast Raman thermometry in driven YBa2Cu3O6.48. Physical Review B, 109(19): 195141. doi:10.1103/PhysRevB.109.195141.

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PhysRevB.109.195141.pdf (Publisher version), 2MB
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Chou_et_al_Supplemental_Material.pdf (Supplementary material), 2MB
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Supplemental Material: provides details of the experimental setup, data processing, extrapolation method for zero-fluence temperatures, deconvolution analysis, and heating calculations.
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https://arxiv.org/abs/2310.00128 (Preprint)
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https://doi.org/10.1103/PhysRevB.109.195141 (Publisher version)
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 Creators:
Chou, T.-H.1, 2, Author           
Först, M.2, Author
Fechner, M.2, Author
Henstridge, M.2, 3, Author
Roy, S.2, Author
Buzzi, M.2, Author
Nicoletti, D.2, Author
Liu, Y.4, Author
Nakata, S.4, Author
Keimer, B.4, Author
Cavalleri, A.2, 5, Author
Affiliations:
1International Max Planck Research School for Ultrafast Imaging & Structural Dynamics (IMPRS-UFAST), Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_2266714              
2Quantum Condensed Matter Dynamics, Condensed Matter Dynamics Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society, ou_1938293              
3SLAC National Accelerator Laboratory, ou_persistent22              
4Max Planck Institute for Solid State Research, ou_persistent22              
5Department of Physics, Clarendon Laboratory, University of Oxford, ou_persistent22              

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 Abstract: Signatures of photoinduced superconductivity have been reported in cuprate materials subjected to a coherent phonon drive. A “cold” superfluid was extracted from the transient Terahertz conductivity and was seen to coexist with “hot” uncondensed quasiparticles, a hallmark of a driven-dissipative system of which the interplay between coherent and incoherent responses is not well understood. Here, time resolved spontaneous Raman scattering was used to probe the lattice temperature in the photoinduced superconducting state of YBa2Cu3O6.48. An increase in lattice temperature of up to 140 K was observed by measuring the time dependent Raman scattering intensity of an undriven “spectator” phonon mode. This value is consistent with the estimated increase in quasiparticle temperature measured under the same excitation conditions. These temperature changes provide quantitative information on the nature of the driven state and its decay, and may suggest a strategy to optimize this effect.

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Language(s): eng - English
 Dates: 2024-04-182023-09-292024-04-222024-05-132024-05-15
 Publication Status: Issued
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 Rev. Type: Peer
 Identifiers: arXiv: 2310.00128
DOI: 10.1103/PhysRevB.109.195141
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Project name : We acknowledge support from the Deutsche Forschungsgemeinschaft (DFG; German Research Foundation) via the excellence cluster “CUI: Advanced Imaging of Matter” (EXC 2056, Project No. 390715994) and the priority program SFB925 (Project No. 170620586).
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Title: Physical Review B
  Abbreviation : Phys. Rev. B
Source Genre: Journal
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Publ. Info: Woodbury, NY : American Physical Society
Pages: - Volume / Issue: 109 (19) Sequence Number: 195141 Start / End Page: - Identifier: ISSN: 1098-0121
CoNE: https://pure.mpg.de/cone/journals/resource/954925225008