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  Tuning superconductivity and spin-vortex instabilities in CaKFe4As4 through in-plane antisymmetric strains

Valadkhani, A., Zúñiga Céspedes, B., Mandloi, S., Xu, M., Schmidt, J., Bud'Ko, S. L., et al. (2024). Tuning superconductivity and spin-vortex instabilities in CaKFe4As4 through in-plane antisymmetric strains. Physical Review B, 109(18): L180503, pp. 1-6. doi:10.1103/PhysRevB.109.L180503.

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 Creators:
Valadkhani, Adrian1, Author
Zúñiga Céspedes, Belén2, Author           
Mandloi , Salony1, Author
Xu, Mingyu1, Author
Schmidt, Juan1, Author
Bud'Ko, Sergey L.1, Author
Canfield, Paul C.1, Author
Valentí, Roser1, Author
Gati, Elena3, Author           
Affiliations:
1External Organizations, ou_persistent22              
2Inorganic Chemistry, Max Planck Institute for Chemical Physics of Solids, Max Planck Society, ou_1863425              
3Physics of Quantum Materials, Max Planck Institute for Chemical Physics of Solids, Max Planck Society, ou_1863462              

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Free keywords: Arsenic compounds, Calcium compounds, Density (optical), Iron compounds, Spin density waves, Spin fluctuations, Strain, Vortex flow, Anti-symmetric, In-plane strains, Lattice strain, Nematics, Noncollinear, Normal state, Spin-density-wave order, Strain response, Vortex crystal, Vortex instability, Iron-based Superconductors
 Abstract: Lattice strains of appropriate symmetry have served as an excellent tool to explore the interaction of superconductivity in the iron-based superconductors with orthorhombic-nematic and stripe spin-density-wave (SSDW) order. In this Letter, we contribute to a broader understanding of the coupling of strain to superconductivity and competing normal-state orders by studying CaKFe4As4 under large, in-plane strains of B1g and B2g symmetry. In contrast to the majority of iron-based superconductors, pure CaKFe4As4 exhibits superconductivity with a relatively high transition temperature of Tc∼35K in proximity of a noncollinear, tetragonal, hedgehog spin-vortex crystal (SVC) order. Through experiments and calculations, we demonstrate an anisotropic in-plane strain response of Tc and the favored SVC configuration in CaKFe4As4. This supports a scenario, in which the change in spin fluctuations dominates the strain response of superconducting Tc. Overall, by suggesting moderate B2g strains as an effective parameter to change the stability of SVC and SSDW, we outline a pathway to a unified phase diagram of iron-based superconductivity. © 2024 authors. Published by the American Physical Society. Published by the American Physical Society under the terms of the "https://creativecommons.org/licenses/by/4.0/"Creative Commons Attribution 4.0 International license. Further distribution of this work must maintain attribution to the author(s) and the published article's title, journal citation, and DOI. Open access publication funded by Max Planck Society.

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Language(s): eng - English
 Dates: 2024-05-082024-05-08
 Publication Status: Issued
 Pages: -
 Publishing info: -
 Table of Contents: -
 Rev. Type: -
 Identifiers: DOI: 10.1103/PhysRevB.109.L180503
 Degree: -

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Title: Physical Review B
  Abbreviation : Phys. Rev. B
Source Genre: Journal
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Publ. Info: Woodbury, NY : American Physical Society
Pages: - Volume / Issue: 109 (18) Sequence Number: L180503 Start / End Page: 1 - 6 Identifier: ISSN: 1098-0121
CoNE: https://pure.mpg.de/cone/journals/resource/954925225008