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  Measuring the 34S and 33S Isotopic Ratios of Volatile Sulfur during Planet Formation

Booth, A. S., Drozdovskaya, M. N., Temmink, M., Nomura, H., Dishoeck, E. F. v., Keyte, L., et al. (2024). Measuring the 34S and 33S Isotopic Ratios of Volatile Sulfur during Planet Formation. ASTROPHYSICAL JOURNAL, 975(1): 72. doi:10.3847/1538-4357/ad7817.

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Measuring the 34S and 33S Isotopic Ratios of Volatile Sulfur during Planet Formation.pdf (beliebiger Volltext), 988KB
 
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 Urheber:
Booth, Alice S., Autor
Drozdovskaya, Maria N., Autor
Temmink, Milou, Autor
Nomura, Hideko, Autor
Dishoeck, Ewine F. van1, Autor           
Keyte, Luke, Autor
Law, Charles J., Autor
Leemker, Margot, Autor
van der Marel, Nienke, Autor
Notsu, Shota, Autor
Oeberg, Karin, Autor
Walsh, Catherine, Autor
Affiliations:
1Infrared and Submillimeter Astronomy, MPI for Extraterrestrial Physics, Max Planck Society, ou_159889              

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Schlagwörter: ASYMMETRIC ICE TRAP; ALMA MOLECULAR INVENTORY; FORMING DISK; COMET 67P/CHURYUMOV-GERASIMENKO; PROTOPLANETARY DISKS; MICROWAVE-SPECTRA; C/O RATIO; HALE-BOPP; FRACTIONATION; CHEMISTRYAstronomy & Astrophysics;
 Zusammenfassung: Stable isotopic ratios constitute powerful tools for unraveling the thermal and irradiation history of volatiles. In particular, we can use our knowledge of the isotopic fractionation processes active during the various stages of star, disk, and planet formation to infer the origins of different volatiles with measured isotopic patterns in our own solar system. Observations of planet-forming disks with the Atacama Large Millimeter/submillimeter Array (ALMA) now readily detect the heavier isotopologues of C, O, and N, while the isotopologue abundances and isotopic fractionation mechanisms of sulfur species are less well understood. Using ALMA observations of the SO and SO2 isotopologues in the nearby, molecule-rich disk around the young star Oph-IRS 48 we present the first constraints on the combined S-32/S-34 and S-32/S-33 isotope ratios in a planet-forming disk. Given that these isotopologues likely originate in relatively warm gas (>50 K), like most other Oph-IRS 48 volatiles, SO is depleted in heavy sulfur, while SO2 is enriched compared to solar system values. However, we cannot completely rule out a cooler gas reservoir, which would put the SO sulfur ratios more in line with comets and other solar system bodies. We also constrain the (SO)-O-18/SO ratio and find the limit to be consistent with solar system values given a temperature of 60 K. Together these observations show that we should not assume solar isotopic values for disk sulfur reservoirs, but additional observations are needed to determine the chemical origin of the abundant SO in this disk, inform on what isotopic fractionation mechanism(s) are at play, and aid in unraveling the history of the sulfur budget during the different stages of planet formation.

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Sprache(n): eng - English
 Datum: 2024-10-25
 Publikationsstatus: Online veröffentlicht
 Seiten: 9
 Ort, Verlag, Ausgabe: -
 Inhaltsverzeichnis: -
 Art der Begutachtung: -
 Identifikatoren: ISI: 001342247100001
DOI: 10.3847/1538-4357/ad7817
 Art des Abschluß: -

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Titel: ASTROPHYSICAL JOURNAL
Genre der Quelle: Zeitschrift
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Ort, Verlag, Ausgabe: TEMPLE CIRCUS, TEMPLE WAY, BRISTOL BS1 6BE, ENGLAND : IOP Publishing Ltd
Seiten: - Band / Heft: 975 (1) Artikelnummer: 72 Start- / Endseite: - Identifikator: ISSN: 0004-637X