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  Local Reaction Kinetics by Imaging: CO Oxidation on Polycrystalline Platinum

Suchorski, Y., Spiel, C., Vogel, D., Drachsel, W., Schlögl, R., & Rupprechter, G. (2010). Local Reaction Kinetics by Imaging: CO Oxidation on Polycrystalline Platinum. ChemPhysChem, 11(15), 3231-3235. doi:10.1002/cphc.201000599.

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Item Permalink: https://hdl.handle.net/11858/00-001M-0000-0010-F4D8-F Version Permalink: https://hdl.handle.net/21.11116/0000-0006-6B7C-8
Genre: Journal Article

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 Creators:
Suchorski, Yuri, Author
Spiel, Christian, Author
Vogel, Diana1, Author           
Drachsel, Wolfgang, Author
Schlögl, Robert1, Author           
Rupprechter, Günther, Author
Affiliations:
1Inorganic Chemistry, Fritz Haber Institute, Max Planck Society, ou_24023              

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Free keywords: oxidation; heterogeneous catalysis; kinetics; reactivity; surface chemistry platinum
 Abstract: The locally resolved kinetics of CO oxidation on individual (111), (110) and (100) domains of a polycrystalline Pt foil were obtained by intensity analysis of video-PEEM images (see picture), and are compared to the global kinetics determined simultaneously by mass spectroscopy. The individual domains behave independently, with the propagating reaction fronts being confined within the grain boundaries.

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Language(s): eng - English
 Dates: 2010-10-25
 Publication Status: Issued
 Pages: -
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 Table of Contents: -
 Rev. Type: Peer
 Identifiers: eDoc: 493308
DOI: 10.1002/cphc.201000599
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Title: ChemPhysChem
Source Genre: Journal
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Publ. Info: Weinheim, Germany : Wiley-VCH
Pages: - Volume / Issue: 11 (15) Sequence Number: - Start / End Page: 3231 - 3235 Identifier: ISSN: 1439-4235
CoNE: https://pure.mpg.de/cone/journals/resource/954925409790