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  Ultrafast electron relaxation dynamics in laser-ionized gases observed with time-resolved THz spectroscopy

Frischkorn, C., Kampfrath, T., Perfetti, L., Tegeder, P., Wolf, M., & Gericke, D. O. (2008). Ultrafast electron relaxation dynamics in laser-ionized gases observed with time-resolved THz spectroscopy. In IEEE Digest: 33rd Int. Conf. on Infrared, Millimeter and Terahertz Waves (IRMMW-THz) (pp. 186-186). New York, NY 10017, USA: IEEE.

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 Urheber:
Frischkorn, Christian1, Autor           
Kampfrath, Tobias1, Autor           
Perfetti, Luca, Autor
Tegeder, Petra, Autor
Wolf, Martin1, Autor           
Gericke, Dirk O., Autor
Affiliations:
1Physical Chemistry, Fritz Haber Institute, Max Planck Society, ou_634546              

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Schlagwörter: -
 Zusammenfassung: Ultrashort broadband THz; pulses are applied to probe the electron dynamics of various gases following ionization by an intense femtosecond laser pulse. The dielectric function of the plasma is found to be Drude-like and yields the temporal evolution of the density and collision rate of the free electrons. The electron decay in a plasma with molecular ions such as O-2(+) is much faster than in monatomic plasmas like Ar+/e(-) due to dissociative recombination which is only possible in molecular plasmas. However, adding a small amount of the electron scavenger SF6 to Ar substantially accelerates the electron decay and enables one to reliably determine the electronic temperature. Furthermore, anomalously high, metal-like electron collision rates are found. Kinetic plasma theory dramatically underestimates these rates pointing towards additional velocity-randomizing processes like collective excitations.

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Sprache(n): eng - English
 Datum: 2008-11-05
 Publikationsstatus: Erschienen
 Seiten: -
 Ort, Verlag, Ausgabe: -
 Inhaltsverzeichnis: -
 Art der Begutachtung: Expertenbegutachtung
 Art des Abschluß: -

Veranstaltung

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Titel: 33rd Int. Conf. on Infrared, Millimeter and Terahertz Waves (IRMMW-THz)
Veranstaltungsort: Pasadena, CA
Start-/Enddatum: 2008-09-15 - 2008-09-19

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Titel: IEEE Digest: 33rd Int. Conf. on Infrared, Millimeter and Terahertz Waves (IRMMW-THz)
Genre der Quelle: Konferenzband
 Urheber:
Affiliations:
Ort, Verlag, Ausgabe: New York, NY 10017, USA : IEEE
Seiten: - Band / Heft: - Artikelnummer: - Start- / Endseite: 186 - 186 Identifikator: ISBN: 978-1-4244-2119-0