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  Comment on “Scanning-probe Raman spectroscopy with single-molecule sensitivity”

Domke, K. F., & Pettinger, B. (2007). Comment on “Scanning-probe Raman spectroscopy with single-molecule sensitivity”. Physical Review B, 75(23): 236401. doi:10.1103/PhysRevB.75.236401.

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Item Permalink: https://hdl.handle.net/11858/00-001M-0000-0011-009C-B Version Permalink: https://hdl.handle.net/21.11116/0000-0007-62F2-9
Genre: Journal Article

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Neacsu_revised.pdf (Any fulltext), 280KB
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737418.pdf (Correspondence), 612KB
 
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 Creators:
Domke, Katrin Friederike1, Author           
Pettinger, Bruno1, Author           
Affiliations:
1Physical Chemistry, Fritz Haber Institute, Max Planck Society, ou_634546              

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Free keywords: carbon; copper compounds; Raman spectra; decomposition
 Abstract: We reinterpret the scanning-probe Raman spectra shown in the paper of Neacsu et al. [Phys. Rev. B 73, 193406 (2006)] and compare it to a variety of single-molecule surface-enhanced Raman studies. The observed blinking behavior and spectral features must be attributed to carbon contaminations rather than to malachite green single molecules, because, under the given experimental conditions, the extremely high-field enhancement of 5x109 will inevitably lead to a quick (photo)decomposition of the adsorbate.

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Language(s): eng - English
 Dates: 2007-06-12
 Publication Status: Issued
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 Rev. Type: Peer
 Identifiers: eDoc: 269395
DOI: 10.1103/PhysRevB.75.236401
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Title: Physical Review B
  Alternative Title : Phys. Rev. B
Source Genre: Journal
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Pages: - Volume / Issue: 75 (23) Sequence Number: 236401 Start / End Page: - Identifier: -