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  Imaging delocalized electron clouds: Photoionization of C-60 in Fourier reciprocal space

Rüdel, A., Hentges, R., Becker, U., Chakraborty, H. S., Madjet, M. E., & Rost, J. M. (2002). Imaging delocalized electron clouds: Photoionization of C-60 in Fourier reciprocal space. Physical Review Letters, 89(12): 125503. doi:10.1103/PhysRevLett.89.125503.

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e125503.pdf (Publisher version), 271KB
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2002
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 Creators:
Rüdel, Andy1, Author           
Hentges, Rainer1, Author           
Becker, Uwe1, Author           
Chakraborty, H. S., Author
Madjet, M. E., Author
Rost, J. M., Author
Affiliations:
1Molecular Physics, Fritz Haber Institute, Max Planck Society, ou_634545              

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Free keywords: CROSS-SECTIONS; GAS-PHASE; OSCILLATIONS; CLUSTERS
 Abstract: The dynamics of the photoionization of the two outermost orbitals of C-60 has been studied in the oscillatory regime from threshold to the carbon K edge. We show that geometrical properties of the fullerene electronic hull, such as its diameter and thickness, are contained in the partial photoionization cross sections by examining ratios of partial cross sections as a function of the photon wave number in the Fourier conjugated space. Evaluated in this unconventional manner pbotoemission data reveal directly the desired spatial information.

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Language(s): eng - English
 Dates: 2002-09-16
 Publication Status: Issued
 Pages: -
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: eDoc: 8387
DOI: 10.1103/PhysRevLett.89.125503
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Title: Physical Review Letters
  Other : Phys. Rev. Lett.
Source Genre: Journal
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Publ. Info: Woodbury, N.Y., etc. : American Physical Society.
Pages: - Volume / Issue: 89 (12) Sequence Number: 125503 Start / End Page: - Identifier: ISSN: 0031-9007
CoNE: https://pure.mpg.de/cone/journals/resource/954925433406