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  c(2 x 2) Water-Hydroxyl Layer on Cu(110): A Wetting Layer Stabilized by Bjerrum Defects

Forster, M., Raval, R., Hodgson, A., Carrasco, J., & Michaelides, A. (2011). c(2 x 2) Water-Hydroxyl Layer on Cu(110): A Wetting Layer Stabilized by Bjerrum Defects. Physical Review Letters, 106: 046103. doi:10.1103/PhysRevLett.106.046103.

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Item Permalink: https://hdl.handle.net/11858/00-001M-0000-0011-2D4F-2 Version Permalink: https://hdl.handle.net/21.11116/0000-0005-F48D-9
Genre: Journal Article

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 Creators:
Forster, Matthew1, Author
Raval, Rasmita1, Author
Hodgson, Andrew1, Author
Carrasco, Javier2, 3, Author           
Michaelides, Angelos2, Author
Affiliations:
1Surface Science Research Centre and Department of Chemistry, University of Liverpool, Oxford Street, Liverpool, L69 3BX, United Kingdom, ou_persistent22              
2London Centre for Nanotechnology and Department of Chemistry, University College London, London WC1E 6BT, United Kingdom, ou_persistent22              
3Theory, Fritz Haber Institute, Max Planck Society, D-14195 Berlin, Germany, ou_634547              

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 Abstract: Understanding the composition and stability of mixed water-hydroxyl layers is a key step in describing
wetting and how surfaces respond to redox processes. Here we show that, instead of forming a complete
hydrogen bonding network, structures containing an excess of water over hydroxyl are stabilized on Cu
(110) by forming a distorted hexagonal network of water-hydroxyl trimers containing Bjerrum defects.
This arrangement maximizes the number of strong bonds formed by water donation to OH and provides
uncoordinated OH groups able to hydrogen bond multilayer water and nucleate growth

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Language(s): eng - English
 Dates: 2010-11-112011-01-242011
 Publication Status: Issued
 Pages: 4
 Publishing info: -
 Table of Contents: -
 Rev. Type: Peer
 Identifiers: DOI: 10.1103/PhysRevLett.106.046103
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Title: Physical Review Letters
Source Genre: Journal
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Publ. Info: Woodbury, N.Y., etc. : American Physical Society.
Pages: - Volume / Issue: 106 Sequence Number: 046103 Start / End Page: - Identifier: ISSN: 0031-9007
CoNE: https://pure.mpg.de/cone/journals/resource/954925433406_1