Coulomb explosion imaging of small organic molecules at LCLS

Erk , Benjamin; Rudenko, Artem; Rolles, Daniel; Rudek, Benedikt; Foucar, Lutz; Epp, Sascha; Cryle, Max; Schlichting, Ilme; Bostedt, Christoph; Schorb, Sebastian; Bozek, John; Rouzee, Arnaud; Hundertmark, Axel; Marchenko, Tatiana; Simon, Mark; Filsinger, Frank; Christensen, Lauge; De, Shankar; Trippel, Sebastian; Wada, Shinichi; Ueda, Kiyoshi; Schröter, Claus; Ullrich, Joachim

doi:10.1088/1742-6596/388/2/022108

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Coulomb explosion imaging of small organic molecules at LCLS

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Erk , Benjamin
Max Planck Advanced Study Group at CFEL;
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

Rudenko, Artem
Max Planck Advanced Study Group at CFEL;
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

Rudek, Benedikt
Max Planck Advanced Study Group at CFEL;
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

Epp, Sascha
Max Planck Advanced Study Group at CFEL;
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

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Filsinger, Frank
Molecular Physics, Fritz Haber Institute, Max Planck Society;

Schröter, Claus
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

Ullrich, Joachim
Max Planck Advanced Study Group at CFEL;
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

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Citation

Erk, B., Rudenko, A., Rolles, D., Rudek, B., Foucar, L., Epp, S., et al. (2012). Coulomb explosion imaging of small organic molecules at LCLS. Journal of Physics: Conference Series, 388(2): 022108. doi:10.1088/1742-6596/388/2/022108.

Cite as: https://hdl.handle.net/11858/00-001M-0000-0010-756A-5

Abstract

Fragmentation of small organic molecules by intense few-femtosecond X-ray free-electron laser pulses has been studied using Coulomb explosion imaging. By measuring kinetic energies and emission angles of the ionic fragments in coincidence, we disentangle different fragmentation pathways, for certain cases can reconstruct molecular geometry at the moment of explosion, and show how it depends on LCLS pulse duration.