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Journal Article

Toward atomic resolution diffractive imaging of isolated molecules with X-ray free-electron lasers

MPS-Authors
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Filsinger,  Frank
Molecular Physics, Fritz Haber Institute, Max Planck Society;
Max Planck Advanced Study Group at CFEL;

Rudenko,  Artem
Max Planck Advanced Study Group at CFEL;
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;
J. R. Macdonald Laboratory, Department of Physics, Kansas State University;

Epp,  Sascha
Max Planck Advanced Study Group at CFEL;
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

Erk,  Benjamin
Deutsches Elektronen-Synchrotron (DESY);
Max Planck Advanced Study Group at CFEL;
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

Foucar,  Lutz
Max Planck Advanced Study Group at CFEL;
Department of Biomolecular Mechanisms, Max Planck Institute for Medical Research, Max Planck Society;

Kühnel,  Kai-Uwe
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

Rudek,  Benedikt
Max Planck Advanced Study Group at CFEL;
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;

Weidenspointner,  Georg
Max Planck Semiconductor Laboratory;
High Energy Astrophysics, MPI for Extraterrestrial Physics, Max Planck Society;

Rolles,  Daniel
Max Planck Advanced Study Group at CFEL;
Deutsches Elektronen-Synchrotron (DESY);
Department of Biomolecular Mechanisms, Max Planck Institute for Medical Research, Max Planck Society;

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arXiv:1403.2553.pdf
(Preprint), 9MB

c4fd00028e.pdf
(Publisher version), 3MB

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Citation

Stern, S., Holmegaard, L., Filsinger, F., Rouzée, A., Rudenko, A., Johnsson, P., et al. (2014). Toward atomic resolution diffractive imaging of isolated molecules with X-ray free-electron lasers. Faraday Discussions, 171, 393-418. doi:10.1039/C4FD00028E.


Cite as: https://hdl.handle.net/11858/00-001M-0000-0019-DB0A-6
Abstract
We give a detailed account of the theoretical analysis and the experimental
results of an x-ray-diffraction experiment on quantum-state selected and
strongly laser-aligned gas-phase ensembles of the prototypical large asymmetric
rotor molecule 2,5-diiodobenzonitrile, performed at the Linac Coherent Light
Source [Phys. Rev. Lett. 112, 083002 (2014)]. This experiment is the first step
toward coherent diffractive imaging of structures and structural dynamics of
isolated molecules at atomic resolution, i. e., picometers and femtoseconds,
using x-ray free-electron lasers.