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Journal Article

Two-dimensional spectral interpretation of time-dependent absorption near laser-coupled resonances

MPS-Authors
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Blättermann,  Alexander
Division Prof. Dr. Thomas Pfeifer, MPI for Nuclear Physics, Max Planck Society;

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Ott,  Christian
Division Prof. Dr. Thomas Pfeifer, MPI for Nuclear Physics, Max Planck Society;

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Kaldun,  Andreas
Division Prof. Dr. Thomas Pfeifer, MPI for Nuclear Physics, Max Planck Society;

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Ding,  Thomas
Division Prof. Dr. Thomas Pfeifer, MPI for Nuclear Physics, Max Planck Society;

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Pfeifer,  Thomas
Division Prof. Dr. Thomas Pfeifer, MPI for Nuclear Physics, Max Planck Society;

External Ressource
Fulltext (public)

1403.2609v1
(Preprint), 2MB

Supplementary Material (public)
There is no public supplementary material available
Citation

Blättermann, A., Ott, C., Kaldun, A., Ding, T., & Pfeifer, T. (2014). Two-dimensional spectral interpretation of time-dependent absorption near laser-coupled resonances. Journal of Physics B, 47(12): 124008. doi:10.1088/0953-4075/47/12/124008.


Cite as: http://hdl.handle.net/11858/00-001M-0000-001A-1E4E-2
Abstract
We demonstrate a two-dimensional time-domain spectroscopy method to extract amplitude and phase modifications of excited atomic states caused by the interaction with ultrashort laser pulses. The technique is based on Fourier analysis of the absorption spectrum of perturbed polarization decay. An analytical description of the method reveals how amplitude and phase information can be directly obtained from measurements. We apply the method experimentally to the helium atom, which is excited by attosecond-pulsed extreme ultraviolet light, to characterize laser-induced couplings of doubly excited states.