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Oxidative coupling reactions for the functionalisation of C–H bonds using oxygen

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Gulzar,  Naeem
Research Department List, Max-Planck-Institut für Kohlenforschung, Max Planck Society;

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Schweitzer-Chaput,  Bertrand
Research Group Klußmann, Max-Planck-Institut für Kohlenforschung, Max Planck Society;

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Klussmann,  Martin
Research Group Klußmann, Max-Planck-Institut für Kohlenforschung, Max Planck Society;

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Citation

Gulzar, N., Schweitzer-Chaput, B., & Klussmann, M. (2014). Oxidative coupling reactions for the functionalisation of C–H bonds using oxygen. Catalysis Science & Technology, 4(9), 2778-2796. doi:10.1039/c4cy00544a.


Cite as: http://hdl.handle.net/11858/00-001M-0000-0024-A69F-8
Abstract
Oxidative coupling reactions enable the direct formation of a new bond from two C–H or heteroatom–H bonds without the need for special activating or leaving groups, and are thus interesting in the context of green chemistry. In order to attain high atom economy and sustainability, it is desirable to conduct these reactions catalytically with oxygen or air as terminal oxidant. Here, a representative overview of such reactions is given, illustrating the substrate scope and the variety of catalyst systems. Additionally, mechanisms and general strategies to utilise oxygen in such reactions are discussed.