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Catalytic Asymmetric Dearomatizing Redox Cross Coupling of Ketones with Aryl Hydrazines Giving 1,4-Diketones

MPS-Authors
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Huang,  Shenlin
Research Department List, Max-Planck-Institut für Kohlenforschung, Max Planck Society;

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Kötzner,  Lisa
Research Department List, Max-Planck-Institut für Kohlenforschung, Max Planck Society;

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De,  Chandra Kanta
Research Department List, Max-Planck-Institut für Kohlenforschung, Max Planck Society;

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List,  Benjamin
Research Department List, Max-Planck-Institut für Kohlenforschung, Max Planck Society;

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Citation

Huang, S., Kötzner, L., De, C. K., & List, B. (2015). Catalytic Asymmetric Dearomatizing Redox Cross Coupling of Ketones with Aryl Hydrazines Giving 1,4-Diketones. Journal of the American Chemical Society, 137(10), 3446-3449. doi:10.1021/ja511200j.


Cite as: http://hdl.handle.net/11858/00-001M-0000-0026-D097-2
Abstract
An asymmetric Brønsted acid catalyzed dearomatizing redox cross coupling reaction has been realized, in which aryl hydrazines react with ketones to deliver 1,4-diketones, bearing an all-carbon quarternary stereocenter in high enantiopurity.