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High Frequency Periodic Forcing of the Oscillatory Catalytic CO Oxidation on Pt (110)

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Beta,  Carsten
Laboratory for Fluid Dynamics, Pattern Formation and Biocomplexity, Max Planck Institute for Dynamics and Self-Organization, Max Planck Society;

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Citation

Bodega, P. S., Kaira, P., Beta, C., Krefting, D., Bauer, D., Mirwald-Schulz, B., et al. (2007). High Frequency Periodic Forcing of the Oscillatory Catalytic CO Oxidation on Pt (110). New Journal of Physics, 9(3), 61-1-61-18. doi:10.1088/1367-2630/9/3/061.


Cite as: https://hdl.handle.net/11858/00-001M-0000-0029-1447-F
Abstract
Resonant periodic forcing is applied to catalytic CO oxidation on platinum (110) in the oscillatory regime. The external parameters are chosen such that the unperturbed system spontaneously develops chemical turbulence. By periodically modulating the CO partial pressure, changes in the spatiotemporal behaviour of the system can be induced: the turbulent behaviour is suppressed and frequency locked patterns with sub-harmonic entrainment develop. A novel gas-driving compressor has been implemented to perform the experimental work.