Monitoring Atomic Cluster Expansion by High-Harmonic Generation

Strelkov, V.; Saalmann, U.; Becker, A.; Rost, J. M.

Item

ITEM ACTIONSEXPORT

Add to Basket

Local TagsRelease HistoryDetailsSummary

Released

Journal Article

Monitoring Atomic Cluster Expansion by High-Harmonic Generation

MPS-Authors

/persons/resource/persons184907

Saalmann, U.
Max Planck Institute for the Physics of Complex Systems, Max Planck Society;

/persons/resource/persons184342

Becker, A.
Max Planck Institute for the Physics of Complex Systems, Max Planck Society;

/persons/resource/persons30956

Rost, J. M.
Max Planck Institute for the Physics of Complex Systems, Max Planck Society;

External Resource

No external resources are shared

Fulltext (restricted access)

There are currently no full texts shared for your IP range.

Fulltext (public)

There are no public fulltexts stored in PuRe

Supplementary Material (public)

There is no public supplementary material available

Citation

Strelkov, V., Saalmann, U., Becker, A., & Rost, J. M. (2011). Monitoring Atomic Cluster Expansion by High-Harmonic Generation. Physical Review Letters, 107(11): 113901.

Cite as: https://hdl.handle.net/11858/00-001M-0000-0029-8C29-C

Abstract

High-harmonic generation is shown to be capable of providing time-resolved information about the particle density of a complex system. As an example, we study numerically high-harmonic generation from expanding xenon clusters in a pump-probe laser scheme, where the pump laser pulse induces the cluster explosion and the probe pulse generates harmonics in the expanding cluster. We show that the high-harmonic spectra characterize the properties of the expanding cluster. Hence, measuring the dependence of the harmonic signal on the pump-probe delay suggests itself as an experimental tool to monitor many-particle dynamics with unique temporal resolution; based on optical measurements, this technique is naturally free from any spatial charge effects.