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Molecular wave-packet dynamics on laser-controlled transition states

MPG-Autoren
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Fischer,  Andreas
Division Prof. Dr. Thomas Pfeifer, MPI for Nuclear Physics, Max Planck Society;

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Gärttner,  Martin
Division Prof. Dr. Christoph H. Keitel, MPI for Nuclear Physics, Max Planck Society,;

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Cörlin,  Philipp
Division Prof. Dr. Thomas Pfeifer, MPI for Nuclear Physics, Max Planck Society;

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Schönwald,  Michael
Division Prof. Dr. Thomas Pfeifer, MPI for Nuclear Physics, Max Planck Society;

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Mizuno,  Tomoya
Division Prof. Dr. Thomas Pfeifer, MPI for Nuclear Physics, Max Planck Society;

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Pfeifer,  Thomas
Division Prof. Dr. Thomas Pfeifer, MPI for Nuclear Physics, Max Planck Society;

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Moshammer,  Robert
Division Prof. Dr. Thomas Pfeifer, MPI for Nuclear Physics, Max Planck Society;

Externe Ressourcen

http://link.aps.org/doi/10.1103/PhysRevA.93.012507
(Verlagsversion)

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1410.8032
(Preprint), 2MB

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Zitation

Fischer, A., Gärttner, M., Cörlin, P., Sperl, A. G., Schönwald, M., Mizuno, T., et al. (2016). Molecular wave-packet dynamics on laser-controlled transition states. Physical Review A, 93(1): 012507. doi:10.1103/PhysRevA.93.012507.


Zitierlink: https://hdl.handle.net/11858/00-001M-0000-0029-C834-0
Zusammenfassung
We present a kinematically complete and time-resolved study of the dissociation dynamics of H 2 + using ultrashort extreme-ultraviolet and near-infrared laser pulses. The reaction kinematics can be controlled by varying the time delay between the two pulses. We demonstrate that a time-dependent laser-dressed potential-energy curve enables the control of the nuclear motion. The dynamics is well reproduced by intuitive semiclassical trajectories on a time-dependent potential curve. From this most fundamental scenario we gain insight in the underlying mechanisms which may be applied as design principles for molecular quantum control, particularly for ultrafast molecular reactions involving the motion of protons.