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Stark Interference of Electric and Magnetic Dipole Transitions in the A - X Band of OH

MPS-Authors
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Schewe,  Hanns Christian
Molecular Physics, Fritz Haber Institute, Max Planck Society;

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Zhang,  Dongdong
Molecular Physics, Fritz Haber Institute, Max Planck Society;

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Meijer,  Gerard
Molecular Physics, Fritz Haber Institute, Max Planck Society;

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Vanhaecke,  Nicolas
Molecular Physics, Fritz Haber Institute, Max Planck Society;
Laboratoire Aimé Cotton, CNRS, Université Paris-Sud, ENS Cachan, Université Paris-Saclay;

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Fulltext (public)

PhysRevLett.116.153001.pdf
(Publisher version), 856KB

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Citation

Schewe, H. C., Zhang, D., Meijer, G., Field, R. W., Sartakov, B. G., Groenenboom, G. C., et al. (2016). Stark Interference of Electric and Magnetic Dipole Transitions in the A - X Band of OH. Physical Review Letters, 116(15): 153001. doi:10.1103/PhysRevLett.116.153001.


Cite as: http://hdl.handle.net/11858/00-001M-0000-002A-509A-B
Abstract
An experimental method is demonstrated that allows determination of the ratio between the electric (E1) and magnetic (M1) transition dipole moments in the A−X band of OH, including their relative sign. Although the transition strengths differ by more than 3 orders of magnitude, the measured M1-to-E1 ratio agrees with the ratio of the ab initio calculated values to within 3%. The relative sign is found to be negative, also in agreement with theory.