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Severe chemical ozone loss inside the Arctic polar vortex during winter 1999-2000 inferred from in situ airborne measurements

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Richard, E. C., Aikin, K. C., Andrews, A. E., Daube, B. C., Gerbig, C., Wofsy, S. C., et al. (2001). Severe chemical ozone loss inside the Arctic polar vortex during winter 1999-2000 inferred from in situ airborne measurements. Geophysical Research Letters, 28(11), 2197-2200. doi:10.1029/2001GL012878.


Cite as: https://hdl.handle.net/11858/00-001M-0000-002A-D648-A
Abstract
Lower stratospheric in situ observations are used to quantify both the accumulated ozone loss and the ozone chemical loss rates in the Arctic polar vortex during the 1999-2000 winter. Multiple long-lived trace gas correlations are used to identify parcels in the inner Arctic vortex whose chemical loss rates are unaffected by extra-vortex intrusions. Ozone-tracer correlations are then used to calculate ozone chemical loss rates. During the late winter the ozone chemical loss rate is found to be -46 +/- 6 (1 sigma) ppbv/day. By mid-March 2000, the accumulated ozone chemical loss is 58 +/- 4 % in the lower stratosphere near 450 K potential temperature (similar to 19 km altitude).