Strongly driven quantum pendulum of the carbonyl sulfide molecule

Trippel, Sebastian; Mullins, Terry; Müller, Nele L. M.; Kienitz, Jens S.; Omiste, Juan J.; Stapelfeldt, Henrik; González-Férez, Rosario; Küpper, Jochen

doi:10.1103/PhysRevA.89.051401

アイテム詳細

登録内容を編集ファイル形式で保存

一時保存へ追加

タグ情報を表示リリース履歴を表示詳細要約

公開

学術論文

Strongly driven quantum pendulum of the carbonyl sulfide molecule

MPS-Authors

/persons/resource/persons195039

Müller, Nele L. M.
Center for Free-Electron Laser Science, DESY, Notkestrasse 85, 22607 Hamburg, Germany;
International Max Planck Research School for Ultrafast Imaging & Structural Dynamics (IMPRS-UFAST), Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society;

External Resource

http://dx.doi.org/10.1103/PhysRevA.89.051401
(出版社版)

https://arxiv.org/abs/1401.6897
(プレプリント)

Fulltext (restricted access)

There are currently no full texts shared for your IP range.

フルテキスト (公開)

PhysRevA.89.051401.pdf
(出版社版), 2MB

付随資料 (公開)

There is no public supplementary material available

引用

Trippel, S., Mullins, T., Müller, N. L. M., Kienitz, J. S., Omiste, J. J., Stapelfeldt, H., González-Férez, R., & Küpper, J. (2014). Strongly driven quantum pendulum of the carbonyl sulfide molecule. Physical Review A, 89(5):. doi:10.1103/PhysRevA.89.051401.

引用: https://hdl.handle.net/11858/00-001M-0000-002A-E909-3

要旨

We demonstrate and analyze a strongly driven quantum pendulum in the angular motion of state-selected and laser-aligned carbonyl sulfide molecules. Raman couplings during the rising edge of a 50-ps laser pulse create a wave packet of pendular states, which propagates in the confining potential formed by the polarizability interaction between the molecule and the laser field. This wave-packet dynamics manifests itself as pronounced oscillations in the degree of alignment with a laser-intensity-dependent period.