Heisenberg dimer single molecule magnets in a strong magnetic field

Efremov, D. V.; Klemm, R. A.

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Heisenberg dimer single molecule magnets in a strong magnetic field

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Efremov, D. V.
Max Planck Institute for the Physics of Complex Systems, Max Planck Society;

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Klemm, R. A.
Max Planck Institute for the Physics of Complex Systems, Max Planck Society;

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Citation

Efremov, D. V., & Klemm, R. A. (2002). Heisenberg dimer single molecule magnets in a strong magnetic field. Physical Review B, 66(17): 174427. Retrieved from http://ojps.aip.org/getabs/servlet/GetabsServlet?prog=normal&id=PRBMDO000066000017174427000001&idtype=cvips&gifs=yes.

Cite as: https://hdl.handle.net/11858/00-001M-0000-002B-36A3-5

Abstract

We calculate the static and dynamic properties of single crystal, single molecule magnets consisting of equal spin S=1/2 or 5/2 dimers. The spins in each dimer interact with each other via the Heisenberg exchange interaction and with the magnetic induction B via the Zeeman interaction, and interdimer interactions are negligible. For antiferromagnetic couplings, the static magnetization and specific heat exhibit interesting low-temperature T and strong B quantum effects. We calculate the frequency spectrum of the Fourier transform of the real part of the time autocorrelation function C-11(t) for arbitrary T, B, and compare our results with those obtained for classical spins. We also calculate the inelastic neutron magnetic dynamical structure factor S(q,omega) at arbitrary T, B.