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Journal Article

Imaging delocalized electron clouds: Photoionization of C-60 in Fourier reciprocal space

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Chakraborty,  H. S.
Max Planck Institute for the Physics of Complex Systems, Max Planck Society;

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Madjet,  M. E.
Max Planck Institute for the Physics of Complex Systems, Max Planck Society;

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Rost,  J. M.
Division Prof. Dr. Joachim H. Ullrich, MPI for Nuclear Physics, Max Planck Society;
Max Planck Institute for the Physics of Complex Systems, Max Planck Society;

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Citation

Rüdel, A., Hentges, R., Becker, U., Chakraborty, H. S., Madjet, M. E., & Rost, J. M. (2002). Imaging delocalized electron clouds: Photoionization of C-60 in Fourier reciprocal space. Physical Review Letters, 89(12): 125503. Retrieved from http://ojps.aip.org/getabs/servlet/GetabsServlet?prog=normal&id=PRLTAO000089000012125503000001&idtype=cvips&gifs=yes.


Cite as: https://hdl.handle.net/11858/00-001M-0000-002B-36ED-1
Abstract
The dynamics of the photoionization of the two outermost orbitals of C-60 has been studied in the oscillatory regime from threshold to the carbon K edge. We show that geometrical properties of the fullerene electronic hull, such as its diameter and thickness, are contained in the partial photoionization cross sections by examining ratios of partial cross sections as a function of the photon wave number in the Fourier conjugated space. Evaluated in this unconventional manner pbotoemission data reveal directly the desired spatial information.