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Mixed valence on a pyrochlore lattice - LiV2O4 as a geometrically frustrated magnet

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Shannon,  N.
Max Planck Institute for the Physics of Complex Systems, Max Planck Society;

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Citation

Shannon, N. (2002). Mixed valence on a pyrochlore lattice - LiV2O4 as a geometrically frustrated magnet. European Physical Journal B, 27(4), 527-540. Retrieved from http://link.springer.de/link/service/journals/10051/bibs/2027004/20270527.htm.


Cite as: http://hdl.handle.net/11858/00-001M-0000-002B-377E-6
Abstract
Above 40 K, the magnetic susceptibility of the heavy Fermion spinel LiV2O4 has many features in common with those of geometrically frustrated magnetic insulators, while its room temperature resistivity comfortably exceeds the Mott-Regel limit. This suggests that local magnetic moments, and the underlying geometry of the pyrochlore lattice, play an important role in determining its magnetic properties. We extend a recently introduced tetragonal mean field theory for insulating pyrochlore antiferromagnets to the case where individual tetrahedra contain spins of different lengths, and use this as a starting point to discuss three different scenarios for magnetic and electronic transitions in LiV2O4.