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Ion mobility separation of deprotonated oligosaccharide isomers – evidence for gas-phase charge migration

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Baldauf,  Carsten
Theory, Fritz Haber Institute, Max Planck Society;

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Hofmann,  Johanna
Molecular Physics, Fritz Haber Institute, Max Planck Society;

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Pagel,  Kevin
Molecular Physics, Fritz Haber Institute, Max Planck Society;
Institut für Chemie und Biochemie der Freien Universität Berlin;

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c6cc06247d-1.pdf
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Citation

Struwe, W. B., Baldauf, C., Hofmann, J., Rudd, P. M., & Pagel, K. (2016). Ion mobility separation of deprotonated oligosaccharide isomers – evidence for gas-phase charge migration. Chemical Communications, 52(83), 12353-12356. doi:10.1039/c6cc06247d.


Cite as: http://hdl.handle.net/11858/00-001M-0000-002C-03C1-2
Abstract
There has been increasing evidence that certain isomeric glycans can be separated efficiently by ion mobility-mass spectrometry when deprotonated ions are analyzed. To better understand the fundamentals behind these separations, we here investigate the impact of ionisation mode and adduct formation using IM-MS, density-functional theory and ab initio molecular dynamics.