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Book Chapter

Stimulated X-ray Raman scattering with free-electron laser sources.


Rolles,  D.
Research Group of Structural Dynamics of (Bio)Chemical Systems, MPI for Biophysical Chemistry, Max Planck Society;

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Rohringer, N., Kimberg, V., Weninger, C., Sanchez-Gonzalez, A., Lutman, A., Maxwell, T., et al. (2016). Stimulated X-ray Raman scattering with free-electron laser sources. In J. Rocca, C. Menoni, & M. Marconi (Eds.), X-Ray Lasers 2014, Proceedings of the 14th International Conference on X-Ray Lasers (pp. 201-207). Cham: Springer. doi: 10.1007/978-3-319-19521-6_26.

Cite as: http://hdl.handle.net/11858/00-001M-0000-002C-0D91-2
Stimulated electronic x-ray Raman scattering is the building block for several proposed x-ray pump probe techniques, that would allow the study of electron dynamics at unprecedented timescales. We present high spectral resolution data on stimulated electronic x-ray Raman scattering in a gas sample of neon using a self-amplified spontaneous emission x-ray free-electron laser. Despite the limited spectral coherence and broad bandwidth of these sources, high-resolution spectra can be obtained by statistical methods, opening the path to coherent stimulated x-ray Raman spectroscopy. An extension of these ideas to molecules and the results of a recent experiment in CO are discussed.