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Toward atomic resolution diffractive imaging of isolated molecules with X-ray free-electron lasers.

MPG-Autoren
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Rolles,  D.
Research Group of Structural Dynamics of (Bio)Chemical Systems, MPI for Biophysical Chemistry, Max Planck Society;

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Zitation

Stern, S., Holmegaard, L., Filsinger, F., Rouzée, A., Rudenko, A., Johnsson, P., et al. (2014). Toward atomic resolution diffractive imaging of isolated molecules with X-ray free-electron lasers. Faraday Discussions, 171, 393-418. doi:10.1039/C4FD00028E.


Zitierlink: http://hdl.handle.net/11858/00-001M-0000-002C-0E91-7
Zusammenfassung
We give a detailed account of the theoretical analysis and the experimental results of an X-ray-diffraction experiment on quantum-state selected and strongly laser-aligned gas-phase ensembles of the prototypical large asymmetric rotor molecule 2,5-diiodobenzonitrile, performed at the Linac Coherent Light Source [Phys. Rev. Lett.112, 083002 (2014)]. This experiment is the first step toward coherent diffractive imaging of structures and structural dynamics of isolated molecules at atomic resolution, i.e., picometers and femtoseconds, using X-ray free-electron lasers.