Toward atomic resolution diffractive imaging of isolated molecules with X-ray 
free-electron lasers.

Stern, S.; Holmegaard, L.; Filsinger, F.; Rouzée, A.; Rudenko, A.; Johnsson, P.; Martin, A. V.; Barty, A.; Bostedt, C.; Bozek, J.; Coffee, R.; Epp, S.; Erk, B.; Foucar, L.; Hartmann, R.; Kimmel, N.; Kühnel, K. U.; Maurer, J.; Messerschmidt, M.; Rudek, B.; Starodub, D.; Thøgersen, J.; Weidenspointner, G.; White, T. A.; Stapelfeldt, H.; Rolles, D.; Chapman, H. N.; Küpper, J.

doi:10.1039/C4FD00028E

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Toward atomic resolution diffractive imaging of isolated molecules with X-ray free-electron lasers.

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Rolles, D.
Research Group of Structural Dynamics of (Bio)Chemical Systems, MPI for Biophysical Chemistry, Max Planck Society;

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引用

Stern, S., Holmegaard, L., Filsinger, F., Rouzée, A., Rudenko, A., Johnsson, P., Martin, A. V., Barty, A., Bostedt, C., Bozek, J., Coffee, R., Epp, S., Erk, B., Foucar, L., Hartmann, R., Kimmel, N., Kühnel, K. U., Maurer, J., Messerschmidt, M., Rudek, B., Starodub, D., Thøgersen, J., Weidenspointner, G., White, T. A., Stapelfeldt, H., Rolles, D., Chapman, H. N., & Küpper, J. (2014). Toward atomic resolution diffractive imaging of isolated molecules with X-ray free-electron lasers. Faraday Discussions, 171, 393-418. doi:10.1039/C4FD00028E.

引用: https://hdl.handle.net/11858/00-001M-0000-002C-0E91-7

要旨

We give a detailed account of the theoretical analysis and the experimental results of an X-ray-diffraction experiment on quantum-state selected and strongly laser-aligned gas-phase ensembles of the prototypical large asymmetric rotor molecule 2,5-diiodobenzonitrile, performed at the Linac Coherent Light Source [Phys. Rev. Lett.112, 083002 (2014)]. This experiment is the first step toward coherent diffractive imaging of structures and structural dynamics of isolated molecules at atomic resolution, i.e., picometers and femtoseconds, using X-ray free-electron lasers.