Mesoscale morphology of airborne core-shell nanoparticle clusters: X-ray laser 
coherent diffraction imaging

Pedersoli, E.; Loh, N. D.; Capotondi, F.; Hampton, C. Y.; Sierra, R. G.; Starodub, D.; Bostedt, C.; Bozek, J.; Nelson, A. J.; Aslam, M.; Li, S.; Dravid, V. P.; Martin, A. V.; Aquila, A.; Barty, A.; Fleckenstein, H.; Gumprecht, L.; Liang, M.; Nass, K.; Schulz, J.; White, T. A.; Coppola, N.; Bajt, S.; Barthelmess, M.; Graafsma, H.; Hirsemann, H.; Wunderer, C; Epp, S. W.; Erk, B.; Rudek, B.; Rudenko, A.; Foucar, L.; Kassemeyer, S.; Lomb, L.; Rolles, D.; Shoeman, R. L.; Steinbrener, J.; Hartmann, R.; Hartmann, A.; Hauser, G.; Holl, P.; Kimmel, N.; Reich, C.; Soltau, H.; Weidenspointner, G.; Benner, W. H.; Farquar, G. R.; Hau-Riege, S. P.; Hunter, M. S.; Ekeberg, T.; Hantke, M.; Maia, F. R. N. C.; Tobias, H. J.; Marchesini, S.; Frank, M.; Strüder, L.; Schlichting, I.; Ullrich, J.; Chapman, H. N.; Bucksbaum, P. H.; Kiskinova, M.; Bogan, M. J.

doi:10.1088/0953-4075/46/16/164033

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Mesoscale morphology of airborne core-shell nanoparticle clusters: X-ray laser coherent diffraction imaging

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Rolles, D.
Research Group of Structural Dynamics of (Bio)Chemical Systems, MPI for Biophysical Chemistry, Max Planck Society;

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引用

Pedersoli, E., Loh, N. D., Capotondi, F., Hampton, C. Y., Sierra, R. G., Starodub, D., Bostedt, C., Bozek, J., Nelson, A. J., Aslam, M., Li, S., Dravid, V. P., Martin, A. V., Aquila, A., Barty, A., Fleckenstein, H., Gumprecht, L., Liang, M., Nass, K., Schulz, J., White, T. A., Coppola, N., Bajt, S., Barthelmess, M., Graafsma, H., Hirsemann, H., Wunderer, C., Epp, S. W., Erk, B., Rudek, B., Rudenko, A., Foucar, L., Kassemeyer, S., Lomb, L., Rolles, D., Shoeman, R. L., Steinbrener, J., Hartmann, R., Hartmann, A., Hauser, G., Holl, P., Kimmel, N., Reich, C., Soltau, H., Weidenspointner, G., Benner, W. H., Farquar, G. R., Hau-Riege, S. P., Hunter, M. S., Ekeberg, T., Hantke, M., Maia, F. R. N. C., Tobias, H. J., Marchesini, S., Frank, M., Strüder, L., Schlichting, I., Ullrich, J., Chapman, H. N., Bucksbaum, P. H., Kiskinova, M., & Bogan, M. J. (2013). Mesoscale morphology of airborne core-shell nanoparticle clusters: X-ray laser coherent diffraction imaging. Journal of Physics B: Atomic, Molecular and Optical Physics, 46(16):. doi:10.1088/0953-4075/46/16/164033.

引用: https://hdl.handle.net/11858/00-001M-0000-002C-0FCE-A

要旨

Unraveling the complex morphology of functional materials like core–shell nanoparticles and its evolution in different environments is still a challenge. Only recently has the single-particle coherent diffraction imaging (CDI), enabled by the ultrabright femtosecond free-electron laser pulses, provided breakthroughs in understanding mesoscopic morphology of nanoparticulate matter. Here, we report the first CDI results for Co@SiO2 core–shell nanoparticles randomly clustered in large airborne aggregates, obtained using the x-ray free-electron laser at the Linac Coherent Light Source. Our experimental results compare favourably with simulated diffraction patterns for clustered Co@SiO2 nanoparticles with ~10 nm core diameter and ~30 nm shell outer diameter, which confirms the ability to resolve the mesoscale morphology of complex metastable structures. The findings in this first morphological study of core–shell nanomaterials are a solid base for future time-resolved studies of dynamic phenomena in complex nanoparticulate matter using x-ray lasers.