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学術論文

Coherent Interaction of Light and Single Molecules in a Dielectric Nanoguide

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Faez,  Sanli
Sandoghdar Division, Max Planck Institute for the Science of Light, Max Planck Society;

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Tuerschmann,  Pierre
Sandoghdar Division, Max Planck Institute for the Science of Light, Max Planck Society;

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Haakh,  Harald R.
Sandoghdar Division, Max Planck Institute for the Science of Light, Max Planck Society;

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Goetzinger,  Stephan
Sandoghdar Division, Max Planck Institute for the Science of Light, Max Planck Society;

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Sandoghdar,  Vahid
Sandoghdar Division, Max Planck Institute for the Science of Light, Max Planck Society;

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引用

Faez, S., Tuerschmann, P., Haakh, H. R., Goetzinger, S., & Sandoghdar, V. (2014). Coherent Interaction of Light and Single Molecules in a Dielectric Nanoguide. Physical Review Letters, 113:. doi:10.1103/PhysRevLett.113.213601.


引用: https://hdl.handle.net/11858/00-001M-0000-002D-647A-4
要旨
Many of the currently pursued experiments in quantum optics would greatly benefit from a strong interaction between light and matter. Here, we present a simple new scheme for the efficient coupling of single molecules and photons. A glass capillary with a diameter of 600 nm filled with an organic crystal tightly guides the excitation light and provides a maximum spontaneous emission coupling factor (beta) of 18% for the dye molecules doped in the organic crystal. A combination of extinction, fluorescence excitation, and resonance fluorescence spectroscopy with microscopy provides high-resolution spatio-spectral access to a very large number of single molecules in a linear geometry. We discuss strategies for exploring a range of quantum-optical phenomena, including polaritonic interactions in a mesoscopic ensemble of molecules mediated by a single mode of propagating photons.