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Carbon nanoarchitectures by design: pre-organizing squaric acid with urea

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Jordan,  Thomas
Nina Fechler, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;

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Antonietti,  Markus
Markus Antonietti, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;

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Fechler,  Nina
Nina Fechler, Kolloidchemie, Max Planck Institute of Colloids and Interfaces, Max Planck Society;

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Citation

Jordan, T., Shalom, M., Antonietti, M., & Fechler, N. (2016). Carbon nanoarchitectures by design: pre-organizing squaric acid with urea. Asia-pacific journal of chemical engineering, 11(6), 866-873. doi:10.1002/apj.2020.


Cite as: http://hdl.handle.net/11858/00-001M-0000-002C-9619-5
Abstract
The synthesis of carbon nanoarchitectures from pre-organized precursor complexes with appropriate bonding patterns, here squaric acid and urea, is described. It is shown that depending on the precursor ratio, different crystal morphologies are formed, which can be transformed into nitrogen-containing carbons with either lamellar or hollow tubelike morphology. It is noted that despite the very different architecture, the composition of the final carbons is always close to a ‘C2N’ stoichiometry.