Chip-Based All-Optical Control of Single Molecules Coherently Coupled to a 
Nanoguide

Tuerschmann, Pierre; Rotenberg, Nir; Renger, Jan; Harder, Irina; Lohse, Olga; Utikal, Tobias; Goetzinger, Stephan; Sandoghdar, Vahid

doi:10.1021/acs.nanolett.7b02033

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Chip-Based All-Optical Control of Single Molecules Coherently Coupled to a Nanoguide

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/persons/resource/persons201216

Tuerschmann, Pierre
Sandoghdar Division, Max Planck Institute for the Science of Light, Max Planck Society;

/persons/resource/persons216332

Rotenberg, Nir
Sandoghdar Division, Max Planck Institute for the Science of Light, Max Planck Society;

/persons/resource/persons201166

Renger, Jan
Sandoghdar Division, Max Planck Institute for the Science of Light, Max Planck Society;

/persons/resource/persons201080

Harder, Irina
Micro- & Nanostructuring, Technology Development and Service Units, Max Planck Institute for the Science of Light, Max Planck Society;

/persons/resource/persons201117

Lohse, Olga
Micro- & Nanostructuring, Technology Development and Service Units, Max Planck Institute for the Science of Light, Max Planck Society;

/persons/resource/persons201220

Utikal, Tobias
Sandoghdar Division, Max Planck Institute for the Science of Light, Max Planck Society;

/persons/resource/persons201072

Goetzinger, Stephan
Sandoghdar Division, Max Planck Institute for the Science of Light, Max Planck Society;

/persons/resource/persons201175

Sandoghdar, Vahid
Sandoghdar Division, Max Planck Institute for the Science of Light, Max Planck Society;

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Citation

Tuerschmann, P., Rotenberg, N., Renger, J., Harder, I., Lohse, O., Utikal, T., et al. (2017). Chip-Based All-Optical Control of Single Molecules Coherently Coupled to a Nanoguide. Nano Letters, 17, 4941-4945. doi:10.1021/acs.nanolett.7b02033.

Cite as: https://hdl.handle.net/21.11116/0000-0000-8594-2

Abstract

The feasibility of many proposals in nano quantum-optics depends on the efficient coupling of photons to individual quantum emitters, the possibility to control this interaction on demand, and the scalability of the experimental platform. To address these issues, we report on chip-based systems made of one-dimensional subwavelength dielectric waveguides (nanoguides) and polycyclic aromatic hydrocarbon molecules. We discuss the design and fabrication requirements, present data on extinction spectroscopy of single molecules coupled to a nanoguide mode, and show how an external optical beam can switch the propagation of light via a nonlinear optical process. The presented architecture paves the way for the investigation of many-body phenomena and polaritonic states and can be readily extended to more complex geometries for the realization of quantum integrated photonic circuits.