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Laser-induced blurring of molecular structure information in high harmonic spectroscopy

MPG-Autoren
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Shaaran,  Tahir
Division Prof. Dr. Christoph H. Keitel, MPI for Nuclear Physics, Max Planck Society;

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Zitation

Risoud, F., Leveque, C., Labeye, M., Caillat, J., Maquet, A., Salieres, P., et al. (2017). Laser-induced blurring of molecular structure information in high harmonic spectroscopy. Scientific Reports, 7: 17302. doi:10.1038/s41598-017-17416-9.


Zitierlink: http://hdl.handle.net/21.11116/0000-0000-BADE-5
Zusammenfassung
High harmonic spectroscopy gives access to molecular structure with Angstrom resolution. Such information is encoded in the destructive interferences occurring between the harmonic emissions from the different parts of the molecule. By solving the time-dependent Schrodinger equation, either numerically or with the molecular strong-field approximation, we show that the electron dynamics in the emission process generally results in a strong spectral smoothing of the interferences, blurring the structural information. However we identify specific generation conditions where they are unaffected. These findings have important consequences for molecular imaging and orbital tomography using high harmonic spectroscopy.