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Gradual pressure-induced change in the magnetic structure of the noncollinear antiferromagnet Mn3Ge

MPG-Autoren
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Sukhanov,  A. S.
Inorganic Chemistry, Max Planck Institute for Chemical Physics of Solids, Max Planck Society;

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Singh,  Sanjay
Inorganic Chemistry, Max Planck Institute for Chemical Physics of Solids, Max Planck Society;

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Caron,  L.
Inorganic Chemistry, Max Planck Institute for Chemical Physics of Solids, Max Planck Society;

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Kumar,  V.
Inorganic Chemistry, Max Planck Institute for Chemical Physics of Solids, Max Planck Society;

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Borrmann,  H.
Horst Borrmann, Chemical Metal Science, Max Planck Institute for Chemical Physics of Solids, Max Planck Society;

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Devi,  P.
Inorganic Chemistry, Max Planck Institute for Chemical Physics of Solids, Max Planck Society;

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Manna,  K.
Inorganic Chemistry, Max Planck Institute for Chemical Physics of Solids, Max Planck Society;

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Felser,  C.
Claudia Felser, Inorganic Chemistry, Max Planck Institute for Chemical Physics of Solids, Max Planck Society;

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Zitation

Sukhanov, A. S., Singh, S., Caron, L., Hansen, T., Hoser, A., Kumar, V., et al. (2018). Gradual pressure-induced change in the magnetic structure of the noncollinear antiferromagnet Mn3Ge. Physical Review B, 97(21): 214402, pp. 1-7. doi:10.1103/PhysRevB.97.214402.


Zitierlink: https://hdl.handle.net/21.11116/0000-0001-93FD-C
Zusammenfassung
By means of powder neutron diffraction we investigate changes in the magnetic structure of the coplanar noncollinear antiferromagnet Mn3Ge caused by an application of hydrostatic pressure up to 5 GPa. At ambient conditions the kagome layers of Mn atoms in Mn3Ge order in a triangular 120 degrees spin structure. Under high pressure the spins acquire a uniform out-of-plane canting, gradually transforming the magnetic texture to a noncoplanar configuration. With increasing pressure the canted structure fully transforms into the collinear ferromagnetic one. We observed that magnetic order is accompanied by a noticeable magnetoelastic effect, namely, spontaneous magnetostriction. The latter induces an in-plane magnetostrain of the hexagonal unit cell at ambient pressure and flips to an out-of-plane strain at high pressures in accordance with the change of the magnetic structure.