English
 
Help Privacy Policy Disclaimer
  Advanced SearchBrowse

Item

ITEM ACTIONSEXPORT

Released

Journal Article

Langevin Approach to Quantum Optics with Molecules

MPS-Authors
/persons/resource/persons223667

Reitz,  Michael
Genes Research Group, Research Groups, Max Planck Institute for the Science of Light, Max Planck Society;

/persons/resource/persons223674

Sommer,  Christian
Genes Research Group, Research Groups, Max Planck Institute for the Science of Light, Max Planck Society;

/persons/resource/persons216190

Genes,  Claudiu
Genes Research Group, Research Groups, Max Planck Institute for the Science of Light, Max Planck Society;

External Resource
Fulltext (restricted access)
There are currently no full texts shared for your IP range.
Fulltext (public)
There are no public fulltexts stored in PuRe
Supplementary Material (public)
There is no public supplementary material available
Citation

Reitz, M., Sommer, C., & Genes, C. (2019). Langevin Approach to Quantum Optics with Molecules. Physical Review Letters, 122: 203602. doi:10.1103/PhysRevLett.122.203602.


Cite as: https://hdl.handle.net/21.11116/0000-0002-1879-C
Abstract
We investigate the interaction between light and molecular systems modeled as quantum emitters coupled to a multitude of vibrational modes via a Holstein-type interaction. We follow a quantum Langevin equations approach that allows for analytical derivations of absorption and fluorescence profiles of molecules driven by classical fields or coupled to quantized optical modes. We retrieve analytical expressions for the modification of the radiative emission branching ratio in the Purcell regime and for the asymmetric cavity transmission associated with dissipative cross talk between upper and lower polaritons in the strong coupling regime. We also characterize the Förster resonance energy transfer process between donor-acceptor molecules mediated by the vacuum or by a cavity mode.