Quantum Langevin approach to cavity quantum electrodynamics with molecules

Reitz, Michael; Sommer, Christian; Genes, Claudiu

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Quantum Langevin approach to cavity quantum electrodynamics with molecules

MPG-Autoren

Reitz, Michael
Genes Research Group, Research Groups, Max Planck Institute for the Science of Light, Max Planck Society;

Sommer, Christian
Genes Research Group, Research Groups, Max Planck Institute for the Science of Light, Max Planck Society;

Genes, Claudiu
Genes Research Group, Research Groups, Max Planck Institute for the Science of Light, Max Planck Society;

Externe Ressourcen

https://arxiv.org/pdf/1811.03442.pdf
(Preprint)

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Zitation

Reitz, M., Sommer, C., & Genes, C. (2018). Quantum Langevin approach to cavity quantum electrodynamics with molecules. arXiv:1812.08592.

Zitierlink: http://hdl.handle.net/21.11116/0000-0002-1879-C

Zusammenfassung

We develop a quantum Langevin equations approach to describe the interaction between light and molecular systems modelled as quantum emitters coupled to a multitude of vibrational modes via a Holstein-type interaction. The formalism allows for analytical derivations of absorption and fluorescence profiles both in the transient and steady state regimes of molecules outside and inside optical cavities. We also derive expressions for the cavity-modified radiative emission branching ratio of a single molecule, cavity transmission in the strong coupling regime and Förster resonance energy transfer between donor-acceptor molecules outside and inside optical cavities.