Deutsch
 
Hilfe Datenschutzhinweis Impressum
  DetailsucheBrowse

Datensatz

DATENSATZ AKTIONENEXPORT
Zur Ablage hinzufügen
  DetailsÜbersicht

Freigegeben
Zeitschriftenartikel

Multiple-orbital effects in laser-induced electron diffraction of aligned molecules

MPG-Autoren
/persons/resource/persons221949

de Giovannini,  U.
Nano-Bio Spectroscopy Group and ETSF, Departamento Fisica de Materiales, Universidad del País Vasco, CSIC-UPV/EHU-MPC;
Theory Group, Theory Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society;

/persons/resource/persons22028

Rubio,  A.
Nano-Bio Spectroscopy Group and ETSF, Departamento Fisica de Materiales, Universidad del País Vasco, CSIC-UPV/EHU-MPC;
Theory Group, Theory Department, Max Planck Institute for the Structure and Dynamics of Matter, Max Planck Society;

Externe Ressourcen

https://dx.doi.org/10.1103/PhysRevA.98.041401
(Verlagsversion)

https://arxiv.org/abs/1905.03596
(Preprint)

Volltexte (beschränkter Zugriff)
Für Ihren IP-Bereich sind aktuell keine Volltexte freigegeben.
Volltexte (frei zugänglich)

PhysRevA.98.041401.pdf
(Verlagsversion), 2MB

1905.03596.pdf
(Preprint), 5MB

Ergänzendes Material (frei zugänglich)
Es sind keine frei zugänglichen Ergänzenden Materialien verfügbar
Zitation

Krečinić, F., Wopperer, P., Frusteri, B., Brauße, F., Brisset, J., de Giovannini, U., et al. (2018). Multiple-orbital effects in laser-induced electron diffraction of aligned molecules. Physical Review A, 98: 041401(R). doi:10.1103/PhysRevA.98.041401.


Zitierlink: https://hdl.handle.net/21.11116/0000-0002-5461-2
Zusammenfassung
Photoelectron angular distributions (PADs) resulting from 800 and 1300 nm strong-field ionization of impulsively aligned CF3I molecules were analyzed using time-dependent density functional theory (TDDFT). The normalized difference between the PADs for aligned and antialigned molecules displays large modulations in the high-energy recollision plateau that are assigned to the diffraction of backscattered photoelectrons. The TDDFT calculations reveal that, in spite of their 2.6 eV energy difference, ionization from the HOMO-1 orbital contributes to the diffraction pattern on the same footing as ionization from the doubly degenerate HOMO orbital.