Time- and angle-resolved photoemission spectroscopy of solids in the extreme 
ultraviolet at 500 kHz repetition rate

Puppin, Michele; Deng, Yunpei; Nicholson, Christopher; Feldl, Johannes; Schröter, Niels; Vita, Hendrik; Kirchmann, P. S.; Monney, Claude; Rettig, Laurenz; Wolf, Martin; Ernstorfer, Ralph

doi:10.1063/1.5081938

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Time- and angle-resolved photoemission spectroscopy of solids in the extreme ultraviolet at 500 kHz repetition rate

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Puppin, Michele
Physical Chemistry, Fritz Haber Institute, Max Planck Society;
Laboratory of Ultrafast Spectroscopy, ISIC, and Lausanne Centre for Ultrafast Science (LACUS), Ecole Polytechnique Federale de Lausanne;

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Deng, Yunpei
Physical Chemistry, Fritz Haber Institute, Max Planck Society;
Paul Scherrer Institute, SwissFEL;

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Nicholson, Christopher
Physical Chemistry, Fritz Haber Institute, Max Planck Society;
Department of Physics, University of Fribourg;

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Feldl, Johannes
Physical Chemistry, Fritz Haber Institute, Max Planck Society;

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Schröter, Niels
Physical Chemistry, Fritz Haber Institute, Max Planck Society;
Paul Scherrer Institute, WSLA/202;

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Vita, Hendrik
Physical Chemistry, Fritz Haber Institute, Max Planck Society;

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Monney, Claude
Physical Chemistry, Fritz Haber Institute, Max Planck Society;
Department of Physics, University of Fribourg;

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Rettig, Laurenz
Physical Chemistry, Fritz Haber Institute, Max Planck Society;

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Wolf, Martin
Physical Chemistry, Fritz Haber Institute, Max Planck Society;

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Ernstorfer, Ralph
Physical Chemistry, Fritz Haber Institute, Max Planck Society;

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1811.06939.pdf
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Citation

Puppin, M., Deng, Y., Nicholson, C., Feldl, J., Schröter, N., Vita, H., et al. (2019). Time- and angle-resolved photoemission spectroscopy of solids in the extreme ultraviolet at 500 kHz repetition rate. Review of Scientific Instruments, 90(02): 023104. doi:10.1063/1.5081938.

Cite as: https://hdl.handle.net/21.11116/0000-0002-99D4-2

Abstract

Time- and angle-resolved photoelectron spectroscopy (trARPES) employing a 500
kHz extreme-ultravioled (XUV) light source operating at 21.7 eV probe photon
energy is reported. Based on a high-power ytterbium laser, optical parametric
chirped pulse amplification (OPCPA), and ultraviolet-driven high-harmonic
generation, the light source produces an isolated high-harmonic with 110 meV
bandwidth and a flux of more than $10^{11}$ photons/second on the sample.
Combined with a state-of-the-art ARPES chamber, this table-top experiment
allows high-repetition rate pump-probe experiments of electron dynamics in
occupied and normally unoccupied (excited) states in the entire Brillouin zone
and with a temporal system response function below 40 fs.