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Heteroepitaxy of Co-Based Heusler Compound/Muscovite for Flexible Spintronics

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Chen,  Yi-Cheng
Inorganic Chemistry, Max Planck Institute for Chemical Physics of Solids, Max Planck Society;

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Markou,  Anastasios
Inorganic Chemistry, Max Planck Institute for Chemical Physics of Solids, Max Planck Society;

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Zhang,  Liguo
Inorganic Chemistry, Max Planck Institute for Chemical Physics of Solids, Max Planck Society;

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Felser,  Claudia
Claudia Felser, Inorganic Chemistry, Max Planck Institute for Chemical Physics of Solids, Max Planck Society;

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引用

Chen, Y.-C., Yen, M., Lai, Y.-H., Markou, A., Zhang, L., Chin, Y.-Y., Lin, H.-J., Chen, C.-T., Felser, C., & Chu, Y.-H. (2019). Heteroepitaxy of Co-Based Heusler Compound/Muscovite for Flexible Spintronics. ACS Applied Materials and Interfaces, 11(38), 35162-35168. doi:10.1021/acsami.9b12219.


引用: https://hdl.handle.net/21.11116/0000-0004-DA4F-F
要旨
Materials with high spin-polarization play an important role in the development of spintronics. Co-based Heusler compounds are a promising candidate for practical applications because of their high Curie temperature and tunable half-metallicity. However, it is a challenge to integrate Heusler compounds into thin film heterostructures because of the lack of control on crystallinity and chemical disorder, critical factors of novel behaviors. Here, muscovite is introduced as a growth substrate to fabricate epitaxial Co2MnGa films with mechanical flexibility. The feature of heteroepitaxy is evidenced by the results of X-ray diffraction and transmission electron microscopy. Moreover, high chemical ordering with superior properties is delivered according to the observation of large Hall conductivity (680 Ω-1 cm-1) and highly saturated magnetic moment (∼3.93 μB/f.u.), matching well with bulk crystals. Furthermore, the excellence of magnetic and electrical properties is retained under the various mechanical bending conditions. Such a result suggests that the development of Co2MnGa/muscovite heteroepitaxy provides not only a pathway to the thin film heterostructure based on high-quality Heusler compounds but also a new aspect of spintronic applications on flexible substrates.