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Chapter model systems in heterogeneous catalysis at the atomic level: a personal view

MPG-Autoren
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Freund,  Hans-Joachim
Chemical Physics, Fritz Haber Institute, Max Planck Society;

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Heyde,  Markus
Chemical Physics, Fritz Haber Institute, Max Planck Society;

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Kuhlenbeck,  Helmut
Chemical Physics, Fritz Haber Institute, Max Planck Society;

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Schmidt,  Thomas
Chemical Physics, Fritz Haber Institute, Max Planck Society;

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Shaikhutdinov,  Shamil K.
Chemical Physics, Fritz Haber Institute, Max Planck Society;

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Zitation

Freund, H.-J., Heyde, M., Kuhlenbeck, H., Nilius, N., Risse, T., Schmidt, T., et al. (2020). Chapter model systems in heterogeneous catalysis at the atomic level: a personal view. Science China Chemistry, 63(4), 426-447. doi:10.1007/s11426-019-9671-0.


Zitierlink: https://hdl.handle.net/21.11116/0000-0005-F380-7
Zusammenfassung
The review presents an overview of studies in the surface science of oxide and related surfaces with an emphasis of the studies performed in the authors’ group. Novel instruments and technique developments, as well as their applications are reported, in an attempt to cover studies on model systems of increasing complexity, including some of the key ingredients of an industrially applied heterogeneous catalyst and its fabrication. The review is intended to demonstrate the power of model studies in understanding heterogeneous catalysis at the atomic level. The studies include those on supported nano-particles, both, prepared in vacuum and from solution, interaction of surfaces and the underlying bulk with molecules from the gas phase, strong metal support interaction, as well as the first attempt to include studies on reactions in confined spaces.