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Allylic Amination of Alkenes with Iminothianthrenes to Afford Alkyl Allylamines

MPS-Authors
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Cheng,  Qiang
Research Department Ritter, Max-Planck-Institut für Kohlenforschung, Max Planck Society;

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Chen,  Junting
Research Department Ritter, Max-Planck-Institut für Kohlenforschung, Max Planck Society;

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Lin,  Songyun
Research Department Ritter, Max-Planck-Institut für Kohlenforschung, Max Planck Society;

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Ritter,  Tobias
Research Department Ritter, Max-Planck-Institut für Kohlenforschung, Max Planck Society;

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Citation

Cheng, Q., Chen, J., Lin, S., & Ritter, T. (2020). Allylic Amination of Alkenes with Iminothianthrenes to Afford Alkyl Allylamines. Journal of the American Chemical Society, 142(41), 17287-17293. doi:10.1021/jacs.0c08248.


Cite as: http://hdl.handle.net/21.11116/0000-0007-6F8B-1
Abstract
Allylic C–H amination is currently accomplished with (sulfon)amides or carbamates. Here we show the first allylic amination that can directly afford alkyl allylamines, enabled by the reactivity of thianthrene-based nitrogen sources that can be prepared from primary amines in a single step.