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Core level photoelectron spectroscopy of heterogeneous reactions at liquid–vapor interfaces: Current status, challenges, and prospects

MPS-Authors
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Dupuy,  Remi
Inorganic Chemistry, Fritz Haber Institute, Max Planck Society;

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Richter,  Clemens
Physical Chemistry, Fritz Haber Institute, Max Planck Society;

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Winter,  Bernd
Molecular Physics, Fritz Haber Institute, Max Planck Society;

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Meijer,  Gerard
Molecular Physics, Fritz Haber Institute, Max Planck Society;

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Schlögl,  Robert
Inorganic Chemistry, Fritz Haber Institute, Max Planck Society;

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Bluhm,  Hendrik
Inorganic Chemistry, Fritz Haber Institute, Max Planck Society;

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5.0036178.pdf
(Publisher version), 5MB

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Citation

Dupuy, R., Richter, C., Winter, B., Meijer, G., Schlögl, R., & Bluhm, H. (2021). Core level photoelectron spectroscopy of heterogeneous reactions at liquid–vapor interfaces: Current status, challenges, and prospects. The Journal of Chemical Physics, 154(6): 060901. doi:10.1063/5.0036178.


Cite as: http://hdl.handle.net/21.11116/0000-0007-F87D-6
Abstract
Liquid–vapor interfaces, particularly those between aqueous solutions and air, drive numerous important chemical and physical processes in the atmosphere and in the environment. X-ray photoelectron spectroscopy is an excellent method for the investigation of these interfaces due to its surface sensitivity, elemental and chemical specificity, and the possibility to obtain information on the depth distribution of solute and solvent species in the interfacial region. In this Perspective, we review the progress that was made in this field over the past decades and discuss the challenges that need to be overcome for investigations of heterogeneous reactions at liquid–vapor interfaces under close-torealistic environmental conditions. We close with an outlook on where some of the most exciting and promising developments might lie in this field