Intermolecular Coulombic Decay in Endohedral Fullerene at the 4d -> 4f Resonance

Obaid, Razib; Xiong, Hui; Augustin, Sven; Schnorr, Kirsten; Ablikim, Utuq; Battistoni, Andrea; Wolf, Thomas J. A.; Bilodeau, Rene C.; Osipov, Timur; Gokhberg, Kirill; Rolles, Daniel; LaForge, Aaron C.; Berrah, Nora

doi:10.1103/PhysRevLett.124.113002

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Intermolecular Coulombic Decay in Endohedral Fullerene at the 4d -> 4f Resonance

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Augustin, Sven
Division Prof. Dr. Thomas Pfeifer, MPI for Nuclear Physics, Max Planck Society;

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Schnorr, Kirsten
Division Prof. Dr. Thomas Pfeifer, MPI for Nuclear Physics, Max Planck Society;

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引用

Obaid, R., Xiong, H., Augustin, S., Schnorr, K., Ablikim, U., Battistoni, A., Wolf, T. J. A., Bilodeau, R. C., Osipov, T., Gokhberg, K., Rolles, D., LaForge, A. C., & Berrah, N. (2020). Intermolecular Coulombic Decay in Endohedral Fullerene at the 4d -> 4f Resonance. Physical Review Letters, 124(11):. doi:10.1103/PhysRevLett.124.113002.

引用: https://hdl.handle.net/21.11116/0000-0008-2082-0

要旨

Interniolecular processes offer unique decay mechanisms for complex systems to internally relax. Here, we report the observation of an intermolecular Coulombic decay channel in an endohedral fullerene, a holmium nitride complex (Ho3N) embedded within a C-80 fullerene, between neighboring holmium ions, and between the holmium complex and the carbon cage. By measuring the ions and the electrons in coincidence after XUV photoabsorption, we can isolate the different decay channels, which are found to be more prevalent relative to intra-atomic Auger decay.